In: Journal of Superconductivity and Novel Magnetism, 2015, vol. 28, no. 4, p. 1231-1236
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In: npj Quantum Materials, 2021, vol. 6, no. 1, p. 12
The interplay of nearly degenerate orders in quantum materials can lead to a myriad of emergent phases. A prominent case is that of the high-Tc cuprates for which the relationship between superconductivity and a short-ranged, incommensurate charge density wave in the CuO2 planes involving the dx2−y2 orbitals (Cu-CDW) is a subject of great current interest. Strong modifications of the...
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The semimetallic or semiconducting nature of the transition metal dichalcogenide 1$T$-TiSe$_2$ remains under debate after many decades mainly due to the fluctuating nature of its 2 x 2 x 2 charge-density-wave (CDW) phase at room- temperature. In this letter, using angle-resolved photoemission spectroscopy, we unambiguously demonstrate that the 1$T$-TiSe$_2$ normal state is semimetallic with ...
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In: Physical Review Materials, 2021, vol. 5, no. 7, p. 074002
We present a combined angle-resolved photoemission spectroscopy and low-energy electron diffraction (LEED) study of the prominent transition metal dichalcogenide IrTe2 upon potassium (K) deposition on its surface. Pristine IrTe2 undergoes a series of charge-ordered phase transitions below room temperature that are characterized by the formation of stripes of Ir dimers of different...
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In: Physical Review B, 2020, vol. 102, no. 19, p. 195103
An antiferromagnetic Hund coupling in multiorbital Hubbard systems induces orbital freezing and an associated superconducting instability, as well as unique composite orders in the case of an odd number of orbitals. While the rich phase diagram of the half-filled three-orbital model has recently been explored in detail, the properties of the doped system remain to be clarified. Here, we...
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In: Applied Physics Letters, 2020, vol. 117, no. 6, p. 062401
The binary compound V3Ga can exhibit two near-equilibrium phases, the A15 structure that is superconducting and the Heusler D03 structure that is semiconducting and antiferromagnetic. Density functional theory calculations show that these two phases are nearly degenerate, being separated in energy by only ±10 meV/atom. Our magnetization measurements on bulk-grown samples show ...
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In: Physical Review B, 2020, vol. 101, no. 21, p. 214523
Bi-based cuprate superconductors are important materials for both fundamental research and applications. As in other cuprates, the superconducting phase in the Bi compounds lies close to an antiferromagnetic phase. Our density functional theory calculations based on the strongly-constrained-and- appropriately-normed exchange correlation functional in ...
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In: Physical Review B, 2020, vol. 101, no. 21, p. 214512
We studied the infrared response of polycrystalline samples of the iron arsenide superconductor (Rb,Cs)Ca2Fe4As4F2 (Rb,Cs-12442), which has a bilayer structure similar to the high-Tc cuprates YBa2Cu3O7 (YBCO) and Bi2Sr2CaCu2O8. The c-axis reflectivity spectra Rc have been derived from the reflectivity spectra of the polycrystalline samples Rpoly and the in-plane spectrum of a corresponding...
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In: Proceedings of the National Academy of Sciences, 2020, vol. 117, no. 12, p. 6409-6416
The role of the crystal lattice for the electronic properties of cuprates and other high-temperature superconductors remains controversial despite decades of theoretical and experimental efforts. While the paradigm of strong electronic correlations suggests a purely electronic mechanism behind the insulator-to-metal transition, recently the mutual enhancement of the electron–electron and the...
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In: Physical Review B, 2020, vol. 101, no. 4, p. 041104
Superconductivity with a remarkably high Tc has recently been found in Sr-doped NdNiO2 thin films. While this system bears strong similarities to the cuprates, some differences, such as a weaker antiferromagnetic exchange coupling and possible high-spin moments on the doped Ni sites have been pointed out. Here, we investigate the effect of Hund coupling and crystal field splitting in a simple...
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