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Ultrafast doublon dynamics in photoexcited $1T$-${\mathrm{TaS}}_{2}$

Ligges, M. ; Avigo, I. ; Gole?, Denis ; Strand, H. ?U.? R. ; Beyazit, Y. ; Hanff, K. ; Diekmann, F. ; Stojchevska, L. ; Kalläne, M. ; Zhou, P. ; Rossnagel, K. ; Eckstein, Martin ; Werner, Philipp ; Bovensiepen, U.

In: Physical Review Letters, 2018, vol. 120, no. 16, p. 166401

Strongly correlated materials exhibit intriguing properties caused by intertwined microscopic interactions that are hard to disentangle in equilibrium. Employing nonequilibrium time-resolved photoemission spectroscopy on the quasi-two- dimensional transition-metal dichalcogenide 1T-TaS2, we identify a spectroscopic signature of doubly occupied sites (doublons) that reflects fundamental Mott...