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Université de Fribourg

X-ray study of structural domains in the near-surface region of SrTiO₃ substrates with Y0.6Pr0.4Ba₂Cu₃O₇/La2/3Ca1/3MnO₃ superlattices grown on top

Hoppler, Justin ; Stahn, J. ; Bouyanfif, Houssny ; Malik, Vivek Kumar ; Patterson, B. D. ; Willmott, P. R. ; Cristiani, G. ; Habermeier, H.-U. ; Bernhard, Christian

In: Physical Review B, 2008, vol. 78, no. 13, p. 134111

We investigated with synchrotron x-ray diffraction and reflectometry the formation of structural domains in the near-surface region of single crystalline SrTiO₃ (001) substrates with Y0.6Pr0.4Ba₂Cu₃O₇/La2/3Ca1/3MnO₃ superlattices grown on top. We find that the antiferrodistortive cubic to tetragonal transition, which occurs at...

Université de Fribourg

X-ray absorption study of the ferromagnetic Cu moment at the ${\mathrm{YBa}}_{2}{\mathrm{Cu}}_{3}{\mathrm{O}}_{7}/{\mathrm{La}}_{2/3}{\mathrm{Ca}}_{1/3}{\mathrm{MnO}}_{3}$ interface and variation of its exchange interaction with the Mn moment

Sen, Kaushik ; Perret, Edith ; Alberca, Aurora ; Uribe-Laverde, Miguel Angel ; Marozau, Ivan ; Yazdi-Rizi, M. ; Mallett, Benjamin P. P. ; Maršík, Premysl ; Piamonteze, C. ; Khaydukov, Yu N. ; Döbeli, Max ; Keller, T. ; Biškup, N. ; Varela, M. ; Vašátko, J. ; Munzar, Dominik ; Bernhard, Christian

In: Physical Review B, 2016, vol. 93, no. 20, p. 205131

With x-ray absorption spectroscopy and polarized neutron reflectometry we studied how the magnetic proximity effect at the interface between the cuprate high-TC superconductor YBa2Cu3O7 (YBCO) and the ferromagnet La2/3Ca1/3MnO3 (LCMO) is related to the electronic and magnetic properties of the LCMO layers. In particular, we explored how the magnitude of the ferromagnetic Cu moment on the YBCO...

Université de Fribourg

X-ray absorption spectroscopy study of the electronic and magnetic proximity effects in ${\mathrm{YBa}}_{2}{\mathrm{Cu}}_{3}{\mathrm{O}}_{7}/{\mathrm{La}}_{2/3}{\mathrm{Ca}}_{1/3}{\mathrm{MnO}}_{3}$ and ${\mathrm{La}}_{2$-${}x}{\mathrm{Sr}}_{x}{\mathrm{CuO}}_{4}/{\mathrm{La}}_{2/3}{\mathrm{Ca}}_{1/3}{\mathrm{MnO}}_{3}$ multilayers

Uribe-Laverde, Miguel Angel ; Das, Saikat ; Sen, Kaushik ; Marozau, Ivan ; Perret, E. ; Alberca, A. ; Heidler, J. ; Piamonteze, C. ; Merz, M. ; Nagel, P. ; Schuppler, S. ; Munzar, Dominik ; Bernhard, Christian

In: Physical Review B, 2014, vol. 90, no. 20, p. 205135

With x-ray absorption spectroscopy we investigated the orbital reconstruction and the induced ferromagnetic moment of the interfacial Cu atoms in YBa2Cu3O7/La2/3Ca1/3MnO3 (YBCO/LCMO) and La2−xSrxCuO4/La2/3Ca1/3MnO3 (LSCO/LCMO) multilayers. We demonstrate that these electronic and magnetic proximity effects are coupled and are common to these cuprate/manganite multilayers. Moreover, we show that...

Université de Fribourg

Two-dimensional confinement of 3d¹ electrons in LaTiO₃/LaAlO₃ multilayers

Seo, S. S. A. ; Han, M. J. ; Hassink, G. W. J. ; Choi, W. S. ; Moon, S. J. ; Kim, J. S. ; Susaki, T. ; Lee, Y. S. ; Yu, Jun ; Bernhard, Christian ; Hwang, H. Y. ; Rijnders, G. ; Blank, D. H. A. ; Keimer, B. ; Noh, T. W.

In: Physical Review Letters, 2010, vol. 104, no. 3, p. 036401

We report spectroscopic ellipsometry measurements of the anisotropy of the interband transitions parallel and perpendicular to the planes of (LaTiO₃)n(LaAlO₃)5 multilayers with n=1–3. These provide direct information about the electronic structure of the two-dimensional (2D) 3d¹ state of the Ti ions. In combination with local density approximation, including a Hubbard U calculation, we...

Université de Fribourg

Transient spin density wave order induced in the normal state of BaFe 2 As 2 by coherent lattice oscillations

Kim, Kyung Wan ; Pashkin, A. ; Schäfer, H. ; Beyer, M. ; Porer, M. ; Wolf, T. ; Bernhard, Christian ; Demsar, J. ; Huber, R. ; Leitenstorfer, A.

In: EPJ Web of Conferences, 2013, vol. 41, p. 03012

We trace the ultrafast dynamics of the spin density wave gap of the pnictide system BaFe2As2 probing resonantly with broadband multi-terahertz pulses. The photoexcitation in the low-temperature ground state leads to a fast suppression of the spin order followed by a slower recovery process. Surprisingly, in the normal state, we observe periodic oscillations of the spin density wave feature at a...

Université de Fribourg

Total Angular Momentum Dichroism of the Terahertz Vortex Beams at the Antiferromagnetic Resonances

Sirenko, Andrei A. ; Marsik, Premysl ; Bugnon, Laurent ; Soulier, Mathias ; Bernhard, Christian ; Stanislavchuk, T. N. ; Xu, Xianghan ; Cheong, S.-W.

In: Physical Review Letters, 2021, vol. 126, no. 15, p. 157401

Terahertz vortex beams with different superposition of the orbital angular momentum $l={\pm}1$, ${\pm}2$, ${\pm}3$, and ${\pm}4$ and spin angular momentum ${\sigma}={\pm}1$ were used to study antiferromagnetic (AFM) resonances in TbFe$_3$(BO$_3$)$_4$ and Ni$_3$TeO$_6$ single crystals. In both materials we observed a strong vortex beam dichroism for the AFM resonances that are split in ...

Université de Fribourg

Terahertz vortex beam as a spectroscopic probe of magnetic excitations

Sirenko, Andrei A. ; Maršík, Premysl ; Bernhard, Christian ; Stanislavchuk, T. N. ; Kiryukhin, V. ; Cheong, S.-W.

In: Physical Review Letters, 2019, vol. 122, no. 23, p. 237401

Circularly polarized light with spin angular momentum is one of the most valuable probes of magnetism. We demonstrate that light beams with orbital angular momentum (OAM), or vortex beams, can also couple to magnetism exhibiting dichroisms in a magnetized medium. Resonant optical absorption in a ferrimagnetic crystal depends strongly on both the handedness of the vortex and the direction of...

Université de Fribourg

Terahertz ellipsometry study of the soft mode behavior in ultrathin SrTiO films

Marsik, Premysl ; Sen, Kaushik ; Khmaladze, Jarji ; Yazdi-Rizi, Meghdad ; Mallett, Benjamin P. P. ; Bernhard, Christian

In: Applied Physics Letters, 2016, vol. 108, no. 5, p. 052901

We present a combined study with time-domain terahertz and conventional far-infrared ellipsometry of the temperature dependent optical response of SrTiO₃thin films (82 and 8.5 nm) that are grown by pulsed-laser deposition on (La0.3Sr0.7) (Al0.65Ta0.35)O₃ (LSAT) substrates. We demonstrate that terahertz ellipsometry is very sensitive to the optical...

Université de Fribourg

Terahertz-driven phonon upconversion in SrTiO 3

Kozina, M. ; Fechner, M. ; Marsik, Premysl ; Driel, T. van ; Glownia, J. M. ; Bernhard, Christian ; Radovic, M. ; Zhu, D. ; Bonetti, S. ; Staub, U. ; Hoffmann, M. C.

In: Nature Physics, 2019, vol. 15, no. 4, p. 387–392

Direct manipulation of the atomic lattice using intense long-wavelength laser pulses has become a viable approach to create new states of matter in complex materials. Conventionally, a high-frequency vibrational mode is driven resonantly by a mid- infrared laser pulse and the lattice structure is modified through indirect coupling of this infrared-active phonon to other, lower-frequency...