Université de Fribourg

Subshell-selective x-ray studies of radiative recombination of ${\mathrm{U}}^{92+}$ ions with electrons for very low relative energies

Banaś, D. ; Pajek, M. ; Surzhykov, A. ; Stöhlker, Th. ; Brandau, C. ; Gumberidze, A. ; Kozhuharov, C. ; Beyer, H. F. ; Böhm, S. ; Bosch, F. ; Czarnota, M. ; Chatterjee, S. ; Dousse, Jean-Claude ; Fritzsche, S. ; Hagmann, S. ; Liesen, D. ; Mokler, P. H. ; Müller, A. ; Kumar, A. ; Reuschl, R. ; Sierpowski, D. ; Spillmann, U. ; Szlachetko, Jakub ; Tashenov, S. ; Trotsenko, S. ; Verma, P. ; Warczak, A.

In: Physical Review A, 2015, vol. 92, no. 3, p. 032710

Radiative recombination (RR) into the K shell and L subshells of U92+ ions interacting with cooling electrons has been studied in an x-ray RR experiment at the electron cooler of the Experimental Storage Ring at GSI. The measured radiative recombination rate coefficients for electron-ion relative energies in the range 0–1000 meV demonstrate the importance of relativistic effects. The...

Université de Fribourg

X-ray two-photon absorption with high fluence XFEL pulses

Hoszowska, Joanna ; Szlachetko, Jakub ; Dousse, Jean-Claude ; Błachucki, W. ; Kayser, Yves ; Milne, Ch. ; Pajek, M. ; Boutet, S. ; Messerschmidt, M. ; Williams, G. ; Chantler, C. T.

In: Journal of Physics: Conference Series, 2015, vol. 635, no. 10, p. 102009

We report on nonlinear interaction of solid Fe with intense femtosecond hard x-ray free-electron laser (XFEL) pulses. The experiment was performed at the CXI end- station of the Linac Coherent Light Source (LCLS) by means of high- resolution x-ray emission spectroscopy. The focused x-ray beam provided extreme fluence of ~10⁵ photons/Ų. Two-photon absorption leading to K-shell hollow atom...

Université de Fribourg

High-energy-resolution grazing emission X-ray fluorescence applied to the characterization of thin Al films on Si

Kayser, Yves ; Szlachetko, Jakub ; Banaś, D. ; Cao, Wei ; Dousse, Jean-Claude ; Hoszowska, Joanna ; Kubala-Kukuś, A. ; Pajek, M.

In: Spectrochimica Acta Part B: Atomic Spectroscopy, 2014, vol. 88, p. 136-149

The grazing emission X-ray fluorescence (GEXRF) technique was applied to the analysis of different Al films, with nominal thicknesses in the range of 1 nm to 150 nm, on Si wafers. In GEXRF the sample volume from which the fluorescence intensity is detected is restricted to a near-surface region whose thickness can be tuned by varying the observation angle. This is possible because of the...

Université de Fribourg

Grazing angle X-ray fluorescence from periodic structures on silicon and silica surfaces

Nowak, Stanislaw H. ; Banaś, D. ; Błachucki, Wojciech Maria ; Cao, Wei ; Dousse, Jean-Claude ; Hönicke, P. ; Hoszowska, Joanna ; Jabłoński, Ł. ; Kayser, Yves ; Kubala-Kukuś, A. ; Pajek, M. ; Reinhardt, F. ; Savu, A.V. ; Szlachetko, Jakub

In: Spectrochimica Acta Part B: Atomic Spectroscopy, 2014, vol. 98, p. 65-75

Various 3-dimensional nano-scaled periodic structures with different configurations and periods deposited on the surface of silicon and silica substrates were investigated by means of the grazing incidence and grazing emission X-ray fluorescence techniques. Apart from the characteristics which are typical for particle- and layer-like samples, the measured angular intensity profiles show...

Université de Fribourg

The electronic structure of matter probed with a single femtosecond hard x-ray pulse

Szlachetko, Jakub ; Milne, a), C. J. ; Hoszowska, Joanna ; Dousse, Jean-Claude ; Błachucki, W. ; Sà, J. ; Kayser, Yves ; Messerschmidt, M. ; Abela, R. ; Boutet, S. ; David, Christian ; Williams, G. ; Pajek, M. ; Patterson, B. D. ; Smolentsev, G. ; Bokhoven, J. A. van ; Nachtegaal, M.

In: Structural Dynamics, 2014, vol. 1, no. 2, p. 021101

Physical, biological, and chemical transformations are initiated by changes in the electronic configuration of the species involved. These electronic changes occur on the timescales of attoseconds (10−18 s) to femtoseconds (10−15 s) and drive all subsequent electronic reorganization as the system moves to a new equilibrium or quasi-equilibrium state. The ability to detect the dynamics of...

Université de Fribourg

Enhanced radiative recombination of U⁹²⁺ ions with cooling electrons for the K-shell

Banaś, D. ; Beyer, H .F. ; Bosch, F. ; Brandau, C. ; Böhm, S. ; Chatterjee, S. ; Czarnota, M. ; Dousse, Jean-Claude ; Gumberidze, A. ; Hagmann, S. ; Kozhuharov, C. ; Liesen, D. ; Mokler, P. H. ; Müller, A. ; Kumar, A. ; Pajek, M. ; Reuschl, R. ; Schmidt, E. W. ; Sierpowski, D. ; Spillmann, U. ; Surzhykov, A. ; Stöhlker, Th. ; Szlachetko, Jakub ; Tashenov, S. ; Trotsenko, S. ; Verma, P. ; Warczak, A.

In: Journal of Physics: Conference Series, 2012, vol. 388, no. 6, p. 062044

Observed enhancement of K-shell radiative recombination (RR) of bare uranium ions with cooling electrons is interpreted in terms of of distant transverse collisions in magnetized electron-cooler plasma described within the semiclassical geometrical model (SGM), which was recently proposed. The Monte Carlo simulations based on the proposed approach explains the enhancement measured in RR of...

Université de Fribourg

Depth profiling of dopants implanted in Si using the synchrotron radiation based high-resolution grazing emission technique

Kayser, Yves ; Banaś, D. ; Cao, Wei ; Dousse, Jean-Claude ; Hoszowska, Joanna ; Jagodziński, P. ; Kavčič, Matjaz ; Kubala-Kukuś, A. ; Nowak, S. ; Pajek, M. ; Szlachetko, Jakub

In: X-Ray Spectrometry, 2012, vol. 41, no. 2, p. 98-104

We report on the surface-sensitive grazing emission X-ray fluorescence technique combined with synchrotron radiation excitation and high-resolution detection to realize depth-profile measurements of Al-implanted Si wafers. The principles of grazing emission measurements as well as the benefits offered by synchrotron sources and wavelength-dispersive detection setups are presented. It is shown...

Université de Fribourg

Depth profiles of Al impurities implanted in Si wafers determined by means of the high-resolution grazing emission X-ray fluorescence technique

Kayser, Yves ; Banaś, D. ; Cao, Wei ; Dousse, Jean-Claude ; Hoszowska, Joanna ; Jagodziński, P. ; Kavčič, Matjaz ; Kubala-Kukuś, A. ; Nowak, S. ; Pajek, M. ; Szlachetko, Jakub

In: Spectrochimica Acta Part B: Atomic Spectroscopy, 2010, p. -

The synchrotron radiation based high-resolution grazing emission X-ray fluorescence (GEXRF) technique was used to extract the distribution of Al ions implanted with a dose of 10¹⁶ atoms/cm² in Si wafers with energies ranging between 1 and 100 keV. The depth distributions of the implanted ions were deduced from the measured angular profiles of the Al-Kα X-ray fluorescence line with...

Université de Fribourg

Observation of ultralow-level Al impurities on a silicon surface by high-resolution grazing emission x-ray fluorescence excited by synchrotron radiation

Kubala-Kukus, A. ; Banas, D. ; Cao, Wei ; Dousse, Jean-Claude ; Hoszowska, Joanna ; Kayser, Yves ; Pajek, M. ; Salomé, M. ; Susini, J. ; Szlachetko, Jakub ; Szlachetko, Monika

In: Physical Review B, 2009, vol. 11, p. 113305

We demonstrate that ultralow-level Al impurities on a silicon surface can be measured by using the high-resolution grazing emission x-ray fluorescence (GEXRF) technique combined with synchrotron-radiation excitation. An Al-impurity level of about 10¹² atoms/cm² was reached by observing the Al Kα x-ray fluorescence in the resonant Raman-scattering background-“free” regime by...

Université de Fribourg

Application of the high-resolution grazing-emission x-ray fluorescence method for impurities control in semiconductor nanotechnology

Szlachetko, Jakub ; Banaś, D. ; Kubala-Kukuś, A. ; Pajek, M. ; Cao, Wei ; Dousse, Jean-Claude ; Hoszowska, Joanna ; Kayser, Yves ; Szlachetko, Monika ; Kavčič, M. ; Salome, M. ; Susini, J.

In: Journal of Applied Physics, 2009, vol. 105, p. 086101

We report on the application of synchrotron radiation based high-resolution grazing-emission x-ray fluorescence (GEXRF) method to measure low-level impurities on silicon wafers. The presented high-resolution GEXRF technique leads to direct detection limits of about 10¹² atoms/cm². The latter can be presumably further improved down to 10⁷ atoms/cm² by combining the synchrotron...

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