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Université de Fribourg

NESSi : The Non-Equilibrium Systems Simulation package

Schüler, Michael ; Golež, Denis ; Murakami, Yuta ; Bittner, Nikolaj ; Herrmann, Andreas ; U.R.Strand, Hugo ; Werner, Philipp ; Eckstein, Martin

In: Computer Physics Communications, 2020, vol. 257, no. 2020, p. 107484

The nonequilibrium dynamics of correlated many-particle systems is of interest in connection with pump–probe experiments on molecular systems and solids, as well as theoretical investigations of transport properties and relaxation processes. Nonequilibrium Green’s functions are a powerful tool to study interaction effects in quantum many-particle systems out of equilibrium, and to extract...

Université de Fribourg

Colloidal gelation, a means to study elasto-capillarity effects in foam

Mikhailovskaya, Alesya ; Trappe, Véronique ; Salonen, Anniina

In: Soft Matter, 2020, vol. 16, no. 9, p. 2249–2255

We explore the evolution of the mechanical properties of a coarsening foam containing colloidal particles that undergo a sol–gel transition in the continuous phase. This enables us to investigate the impact of elasto-capillarity on foam mechanics over a wide range of elasto-capillary numbers. Right after initiating aggregation the foam mechanics is predominantly determined by the elasticity...

Université de Fribourg

Colloidal transformations in ms2 virus particles: driven by ph, influenced by natural organic matter

Watts, Samuel ; Julian, Timothy R. ; Maniura-Weber, Katharina ; Graule, Thomas ; Salentinig, Stefan

In: ACS Nano, 2020, vol. 14, no. 2, p. 1879–1887

Enteric viruses, such as enterovirus, norovirus, and rotavirus, are among the leading causes of disease outbreaks due to contaminated drinking and recreational water. Viruses are difficult to remove from water through filtration based on physical size exclusion—for example by gravity-driven filters—due to their nanoscale size. To understand virus removal in drinking water treatment ...

Université de Fribourg

Colloidal dynamics and elasticity of dense wax particle suspensions over a wide range of volume fractions when tuning the softness by temperature

Yoon, Jiwon ; Scheffold, Frank ; Ahn, Kyung Hyun

In: Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2019, vol. 576, p. 1–8

We report on the colloidal dynamics and rheology of liquid droplet emulsions and solid particle suspensions over a wide range of volume fractions. Diffusing wave spectroscopy and rheometry were utilized to study the micro/macroscale properties of 1-eicosene wax particles dispersed in water. By changing the temperature, the wax droplets change their properties from soft to hard or vice versa,...

Université de Fribourg

Robust equilibria in location games

Buechel, Berno ; Roehl, Nils

In: European Journal of Operational Research, 2015, vol. 240, no. 2, p. 505-517

In the framework of spatial competition, two or more players strategically choose a location in order to attract consumers. It is assumed standardly that consumers with the same favorite location fully agree on the ranking of all possible locations. To investigate the necessity of this questionable and restrictive assumption, we model heterogeneity in consumers’ distance perceptions by...

Université de Fribourg

Supramolecular structures in lipid digestion and implications for functional food delivery

Salentinig, Stefan

In: Current Opinion in Colloid & Interface Science, 2019, vol. 39, p. 190–201

The daily diet is important for our survival, health, and wellbeing. Functional food materials, which tailor the digestion process, can help maintaining and even improving human health and lifestyle. Knowledge on how food products, particularly food emulsions such as milk, interact with the digestive system, where they transform into supramolecular structures, can have a direct impact on the...

Université de Fribourg

Observation of strongly heterogeneous dynamics at the depinning transition in a colloidal glass

Şenbil, Nesrin ; Gruber, Markus ; Zhang, Chi ; Fuchs, Matthias ; Scheffold, Frank

In: Physical Review Letters, 2019, vol. 122, no. 10, p. 108002

We study experimentally the origin of heterogeneous dynamics in strongly driven glass-forming systems. Thereto, we apply a well-defined force with a laser line trap on individual colloidal polystyrene probe particles seeded in an emulsion glass composed of droplets of the same size. Fluid and glass states can be probed. We monitor the trajectories of the probe and measure displacements and...

Université de Fribourg

Diffusing wave microrheology of highly scattering concentrated monodisperse emulsions

Kim, Ha Seong ; Şenbil, Nesrin ; Zhang, Chi ; Scheffold, Frank ; Mason, Thomas G.

In: Proceedings of the National Academy of Sciences, 2019, vol. 116, no. 16, p. 7766–7771

Motivated by improvements in diffusing wave spectroscopy (DWS) for nonergodic, highly optically scattering soft matter and by cursory treatment of collective scattering effects in prior DWS microrheology experiments, we investigate the low-frequency plateau elastic shear moduli G′p of concentrated, monodisperse, disordered oil-in- water emulsions as droplets jam. In such experiments, the...

Université de Fribourg

Effect of clustering on the heat generated by superparamagnetic iron oxide nanoparticles

Lattuada, Marco

In: CHIMIA International Journal for Chemistry, 2019, vol. 73, no. 1, p. 39–42

Magnetic nanoparticles have been the subject of enormous investigations for their potential use as cancer treatment via hyperthermia. This is due to their ability to generate heat when exposed to an external magnetic field oscillating at sufficiently high frequency. There are many different parameters that need to be considered when designing the optimal nanoparticle formulation for...