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Université de Fribourg

Nonthermal excitonic condensation near a spin-state transition

Werner, Philipp ; Murakami, Yuta

In: Physical Review B, 2020, vol. 102, no. 2020-24, p. 241103

Recent experiments demonstrate the induction of long-range order in correlated electron systems via external perturbations, which calls for a better understanding of nonthermal ordered states and nonequilibrium symmetry breaking. Here, we reveal a mechanism based on entropy cooling and entropy trapping in a strongly correlated multiorbital system. We consider a two-orbital Hubbard model with...

Université de Fribourg

How circular dichroism in time- and angle-resolved photoemission can be used to spectroscopically detect transient topological states in graphene

Schüler, Michael ; Giovannini, Umberto De ; Hübener, Hannes ; Rubio, Angel ; Sentef, Michael A. ; Devereaux, Thomas P. ; Werner, Philipp

In: Physical Review X, 2020, vol. 10, no. 4, p. 041013

Pumping graphene with circularly polarized light is the archetype of light-tailoring topological bands. Realizing the induced Floquet-Chern-insulator state and demonstrating clear experimental evidence for its topological nature has been a challenge, and it has become clear that scattering effects play a crucial role. We tackle this gap between theory and experiment by employing microscopic...

Université de Fribourg

Photoenhanced excitonic correlations in a Mott insulator with nonlocal interactions

Bittner, Nikolaj ; Golež, Denis ; Eckstein, Martin ; Werner, Philipp

In: Physical Review B, 2020, vol. 101, no. 8, p. 085127

We investigate the effect of nonlocal interactions on the photodoped Mott insulating state of the two-dimensional Hubbard model using a nonequilibrium generalization of the dynamical cluster approximation. In particular, we compare the situation where the excitonic states are lying within the continuum of doublon-holon excitations to a setup where the excitons appear within the Mott gap. In...

Université de Fribourg

Local Berry curvature signatures in dichroic angle-resolved photoelectron spectroscopy from two-dimensional materials

Schüler, Michael ; Giovannini, Umberto De ; Hübener, Hannes ; Rubio, Angel ; Sentef, Michael A. ; Werner, Philipp

In: Science Advances, 2020, vol. 6, no. 9, p. eaay2730

Topologically nontrivial two-dimensional materials hold great promise for next- generation optoelectronic applications. However, measuring the Hall or spin-Hall response is often a challenge and practically limited to the ground state. An experimental technique for tracing the topological character in a differential fashion would provide useful insights. In this work, we show that circular...

Université de Fribourg

Electron–phonon-driven three-dimensional metallicity in an insulating cuprate

Baldini, Edoardo ; Sentef, Michael A. ; Acharya, Swagata ; Brumme, Thomas ; Sheveleva, Evgeniia ; Lyzwa, Fryderyk ; Pomjakushina, Ekaterina ; Bernhard, Christian ; van Schilfgaarde, Mark ; Carbone, Fabrizio ; Rubio, Angel ; Weber, Cédric

In: Proceedings of the National Academy of Sciences, 2020, vol. 117, no. 12, p. 6409-6416

The role of the crystal lattice for the electronic properties of cuprates and other high-temperature superconductors remains controversial despite decades of theoretical and experimental efforts. While the paradigm of strong electronic correlations suggests a purely electronic mechanism behind the insulator-to-metal transition, recently the mutual enhancement of the electron–electron and the...

Université de Fribourg

Ultrafast nonequilibrium evolution of excitonic modes in semiconductors

Murakami, Yuta ; Schüler, Michael ; Takayoshi, Shintaro ; Werner, Philipp

In: Physical Review B, 2020, vol. 101, no. 3, p. 035203

We study the time evolution of excitonic states after photoexcitation in the one- dimensional spinless extended Falicov-Kimball model. Several numerical methods are employed and benchmarked against each other: time-dependent mean-field simulations, the second-Born approximation (2BA) within the Kadanoff-Baym formalism, the generalized Kadanoff-Baym ansatz (GKBA) implemented with the 2BA, and...

Université de Fribourg

Classification and characterization of nonequilibrium Higgs modes in unconventional superconductors

Schwarz, L. ; Fauseweh, B. ; Tsuji, N. ; Cheng, N. ; Bittner, Nikolaj ; Krull, H. ; Berciu, M. ; Uhrig, G.S. ; Schnyder, A.P. ; Kaiser, S. ; Manske, D.

In: Nature Communications, 2020, vol. 11, no. 1, p. 1–9

Recent findings of new Higgs modes in unconventional superconductors require a classification and characterization of the modes allowed by nontrivial gap symmetry. Here we develop a theory for a tailored nonequilibrium quantum quench to excite all possible oscillation symmetries of a superconducting condensate. We show that both a finite momentum transfer and quench symmetry allow for an...

Université de Fribourg

Adiabatic preparation of a correlated symmetry‐broken initial state with the generalized Kadanoff–Baym Ansatz

Tuovinen, Riku ; Golež, Denis ; Schüler, Michael ; Werner, Philipp ; Eckstein, Martin ; Sentef, Michael A.

In: physica status solidi (b), 2019, vol. 256, no. 7, p. 1800469

A fast time propagation method for nonequilibrium Green's functions (NEGF) based on the generalized Kadanoff–Baym Ansatz (GKBA) is applied to a lattice system with a symmetry‐broken equilibrium phase, namely an excitonic insulator (EI). The adiabatic preparation of a correlated symmetry‐broken initial state from a Hartree– Fock wave function within GKBA is assessed by comparing with a...

Université de Fribourg

Excited-state band mapping and momentum-resolved ultrafast population dynamics in In/Si(111) nanowires investigated with XUV-based time- and angle-resolved photoemission spectroscopy

Nicholson, Christopher W. ; Puppin, M. ; Lücke, A. ; Gerstmann, U. ; Krenz, M. ; Schmidt, W. G. ; Rettig, L. ; Ernstorfer, R. ; Wolf, M.

In: Physical Review B, 2019, vol. 99, no. 15, p. 155107

We investigate the excited state electronic structure of the model phase transition system In/Si(111) using femtosecond time- and angle-resolved photoemission spectroscopy (trARPES). An extreme ultraviolet 500 kHz laser source at 21.7 eV is utilized both to map the energy of excited states above the Fermi level and follow the momentum-resolved population dynamics on a femtosecond timescale....

Université de Fribourg

Terahertz-driven phonon upconversion in SrTiO 3

Kozina, M. ; Fechner, M. ; Marsik, Premysl ; Driel, T. van ; Glownia, J. M. ; Bernhard, Christian ; Radovic, M. ; Zhu, D. ; Bonetti, S. ; Staub, U. ; Hoffmann, M. C.

In: Nature Physics, 2019, vol. 15, no. 4, p. 387–392

Direct manipulation of the atomic lattice using intense long-wavelength laser pulses has become a viable approach to create new states of matter in complex materials. Conventionally, a high-frequency vibrational mode is driven resonantly by a mid- infrared laser pulse and the lattice structure is modified through indirect coupling of this infrared-active phonon to other, lower-frequency...