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Université de Fribourg

Probing the interplay between lattice dynamics and short-range magnetic correlations in CuGeO3 with femtosecond RIXS

Paris, E. ; Nicholson, Christopher W. ; Johnston, S. ; Tseng, Y. ; Rumo, Maxime ; Coslovich, G. ; Zohar, S. ; Lin, M. F. ; Strocov, V. N. ; Saint-Martin, R. ; Revcolevschi, A. ; Kemper, A. ; Schlotter, W. ; Dakovski, G. L. ; Monney, Claude ; Schmitt, T.

In: npj Quantum Materials, 2021, vol. 6, no. 1, p. 51

Investigations of magnetically ordered phases on the femtosecond timescale have provided significant insights into the influence of charge and lattice degrees of freedom on the magnetic sub-system. However, short-range magnetic correlations occurring in the absence of long-range order, for example in spin-frustrated systems, are inaccessible to many ultrafast techniques. Here, we show how...

Université de Fribourg

Nonthermal excitonic condensation near a spin-state transition

Werner, Philipp ; Murakami, Yuta

In: Physical Review B, 2020, vol. 102, no. 2020-24, p. 241103

Recent experiments demonstrate the induction of long-range order in correlated electron systems via external perturbations, which calls for a better understanding of nonthermal ordered states and nonequilibrium symmetry breaking. Here, we reveal a mechanism based on entropy cooling and entropy trapping in a strongly correlated multiorbital system. We consider a two-orbital Hubbard model with...

Université de Fribourg

Nature of native atomic defects in ${\mathrm{ZrTe}}_{5}$ and their impact on the low-energy electronic structure

Salzmann, Björn ; Pulkkinen, Aki ; Hildebrand, Baptiste ; Jaouen, Thomas ; Zhang, S. N. ; Martino, E. ; Li, Q. ; Gu, G. ; Berger, Helmuth ; Yazyev, O. V. ; Akrap, Ana ; Monney, Claude

In: Physical Review Materials, 2020, vol. 4, no. 11, p. 114201

Over the past decades, investigations of the anomalous low-energy electronic properties of ZrTe5 have reached a wide array of conclusions. An open question is the growth method's impact on the stoichiometry of ZrTe5 samples, especially given the very small density of states near its chemical potential. Here we report on high- resolution scanning tunneling microscopy and spectroscopy...

Université de Fribourg

Mapping the unoccupied state dispersions in ${\mathrm{Ta}}_{2}{\mathrm{NiSe}}_{5}$ with resonant inelastic x-ray scattering

Monney, Claude ; Herzog, Marc ; Pulkkinen, Aki ; Huang, Y. ; Pelliciari, Jonathan ; Olalde-Velasco, P. ; Katayama, Naoyuk ; Nohara, Minoru ; Takagi, Hide ; Schmitt, Thorsten ; Mizokawa, Takashi

In: Physical Review B, 2020, vol. 102, no. 8, p. 085148

The transition metal chalcogenide Ta2NiSe5 undergoes a second-order phase transition at Tc=328K involving a small lattice distortion. Below Tc, a band gap at the center of its Brillouin zone increases up to about 0.35 eV. In this work, we study the electronic structure of Ta2NiSe5 in its low-temperature semiconducting phase, using resonant inelastic x-ray scattering (RIXS) at the Ni L3 edge....

Université de Fribourg

Examining the surface phase diagram of ${\mathrm{IrTe}}_{2}$ with photoemission

Rumo, Maxime ; Nicholson, Christopher W. ; Pulkkinen, Aki ; Hildebrand, Baptiste ; Kremer, Geoffroy ; Salzmann, Björn ; Mottas, Marie-Laure ; Ma, K. Y. ; Wong, E. L. ; Man, M. K. L. ; Dani, K. M. ; Barbiellini, B. ; Muntwiler, Matthias ; Jaouen, Thomas ; Rohr, F. O. von ; Monney, Claude

In: Physical Review B, 2020, vol. 101, no. 23, p. 235120

In the transition metal dichalcogenide IrTe2, low-temperature charge-ordered phase transitions involving Ir dimers lead to the occurrence of stripe phases of different periodicities, and nearly degenerate energies. Bulk-sensitive measurements have shown that, upon cooling, IrTe2 undergoes two such first-order transitions to (5×1×5) and (8×1×8) reconstructed phases at Tc1∼280 K and...

Université de Fribourg

Collective modes in excitonic insulators: Effects of electron-phonon coupling and signatures in the optical response

Murakami, Yuta ; Golež, Denis ; Kaneko, Tatsuya ; Koga, Akihisa ; Millis, Andrew J. ; Werner, Philipp

In: Physical Review B, 2020, vol. 101, no. 19, p. 195118

We consider a two-band spinless model describing an excitonic insulator (EI) on the two-dimensional square lattice with anisotropic hopping parameters and electron-phonon (el-ph) coupling, inspired by the EI candidate Ta2NiSe5. We systematically study the nature of the collective excitations in the ordered phase which originates from the interband Coulomb interaction and the el-ph coupling. ...

Université de Fribourg

Ultrafast nonequilibrium evolution of excitonic modes in semiconductors

Murakami, Yuta ; Schüler, Michael ; Takayoshi, Shintaro ; Werner, Philipp

In: Physical Review B, 2020, vol. 101, no. 3, p. 035203

We study the time evolution of excitonic states after photoexcitation in the one- dimensional spinless extended Falicov-Kimball model. Several numerical methods are employed and benchmarked against each other: time-dependent mean-field simulations, the second-Born approximation (2BA) within the Kadanoff-Baym formalism, the generalized Kadanoff-Baym ansatz (GKBA) implemented with the 2BA, and...

Université de Fribourg

Role of a higher-dimensional interaction in stabilizing charge density waves in quasi-one-dimensional ${\mathrm{NbSe}}_{3}$ revealed by angle-resolved photoemission spectroscopy

Nicholson, Christopher W. ; Schwier, Eike Fabian ; Shimada, K. ; Berger, Helmuth ; Hoesch, M. ; Berthod, C. ; Monney, Claude

In: Physical Review B, 2020, vol. 101, no. 4, p. 045412

We revisit charge density wave (CDW) behavior in the archetypal quasi-one- dimensional (quasi-1D) material NbSe3 by high-resolution angle-resolved photoemission spectroscopy measurements utilizing a microfocused laser with a photon energy of 6.3 eV. We present a detailed view of the electronic structure of this complex multiband system and unambiguously resolve CDW gaps at the Fermi level ...

Université de Fribourg

Real- and Q-space travelling: multi-dimensional distribution maps of crystal-lattice strain (∊044) and tilt of suspended monolithic silicon nanowire structures

Dolabella, Simone ; Frison, Ruggero ; Chahine, Gilbert A. ; Richter, Carsten ; Schulli, Tobias U. ; Tasdemir, Zuhal ; Alaca, B. Erdem ; Leblebic, Yusuf ; Dommann, Alex ; Neels, Antonia

In: Journal of Applied Crystallography, 2020, vol. 53, no. 1, p. 58–68

Silicon nanowire-based sensors find many applications in micro- and nano- electromechanical systems, thanks to their unique characteristics of flexibility and strength that emerge at the nanoscale. This work is the first study of this class of micro- and nano-fabricated silicon-based structures adopting the scanning X-ray diffraction microscopy technique for mapping the in-plane crystalline...