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Randomization and the Gross-Pitaevskii Hierarchy

Sohinger, Vedran ; Staffilani, Gigliola

In: Archive for Rational Mechanics and Analysis, 2015, vol. 218, no. 1, p. 417-485

Université de Fribourg

Mapping the unoccupied state dispersions in ${\mathrm{Ta}}_{2}{\mathrm{NiSe}}_{5}$ with resonant inelastic x-ray scattering

Monney, Claude ; Herzog, Marc ; Pulkkinen, Aki ; Huang, Y. ; Pelliciari, Jonathan ; Olalde-Velasco, P. ; Katayama, Naoyuk ; Nohara, Minoru ; Takagi, Hide ; Schmitt, Thorsten ; Mizokawa, Takashi

In: Physical Review B, 2020, vol. 102, no. 8, p. 085148

The transition metal chalcogenide Ta2NiSe5 undergoes a second-order phase transition at Tc=328K involving a small lattice distortion. Below Tc, a band gap at the center of its Brillouin zone increases up to about 0.35 eV. In this work, we study the electronic structure of Ta2NiSe5 in its low-temperature semiconducting phase, using resonant inelastic x-ray scattering (RIXS) at the Ni L3 edge....

Université de Fribourg

Simple and fast evaluation of relaxation parameters of magnetic nanoparticles

Lemal, Philipp ; Balog, Sandor ; Ackermann-Hirschi, Liliane ; Taladriz-Blanco, Patricia ; Hirt, Ann M. ; Rothen-Rutishauser, Barbara ; Lattuada, Marco ; Petri-Fink, Alke

In: Journal of Magnetism and Magnetic Materials, 2020, vol. 499, p. 166176

The efficacy of magnetic hyperthermia treatment depends on the optimal available magnetic nanoparticles (MNPs) that are excited in a given alternating magnetic field and viscosity of the region of interest. In this regard, assessing the relevant relaxation parameters is of upmost importance and could improve the speed of development of efficient applications. Here, we demonstrate how to...

Université de Fribourg

Coupling of electronic and nuclear motion in a negative ion resonance: Experimental and theoretical study of benzene

Allan, Michael ; Čurík, Roman ; Čársky, Petr

In: The Journal of Chemical Physics, 2019, vol. 151, no. 6, p. 064119

We present calculated and measured elastic and vibrational excitation cross sections in benzene with the objective to assess the reliability of the theoretical method and to shed more light on how the electronic motion of the incoming electron is coupled with the nuclear motion of the vibrations. The calculation employed the discrete momentum representation method which involves solving the...

Université de Fribourg

Terahertz vortex beam as a spectroscopic probe of magnetic excitations

Sirenko, Andrei A. ; Maršík, Premysl ; Bernhard, Christian ; Stanislavchuk, T. N. ; Kiryukhin, V. ; Cheong, S.-W.

In: Physical Review Letters, 2019, vol. 122, no. 23, p. 237401

Circularly polarized light with spin angular momentum is one of the most valuable probes of magnetism. We demonstrate that light beams with orbital angular momentum (OAM), or vortex beams, can also couple to magnetism exhibiting dichroisms in a magnetized medium. Resonant optical absorption in a ferrimagnetic crystal depends strongly on both the handedness of the vortex and the direction of...

Université de Fribourg

Highly elastic polyrotaxane binders for mechanically stable lithium hosts in lithium‐metal batteries

Yoo, Dong‐Joo ; Elabd, Ahmed ; Choi, Sunghun ; Cho, Yunshik ; Kim, Jaemin ; Lee, Seung Jong ; Choi, Seung Ho ; Kwon, Tae‐woo ; Char, Kookheon ; Kim, Ki Jae ; Coskun, Ali ; Choi, Jang Wook

In: Advanced Materials, 2019, vol. 31, no. 29, p. 1901645

Despite their unparalleled theoretical capacity, lithium‐metal anodes suffer from well‐ known indiscriminate dendrite growth and parasitic surface reactions. Conductive scaffolds with lithium uptake capacity are recently highlighted as promising lithium hosts, and carbon nanotubes (CNTs) are an ideal candidate for this purpose because of their capability of percolating a conductive...

Université de Fribourg

Laboratory based XAS measurements, electron-induced double K-shell ionization of Sc, Cr and Cu : and, Chemical sensitivity of photoinduced Kʰβ hypersatelite transition in Cr compounds

Zeeshan, Faisal ; Dousse, Jean-Claude (Dir.)

Thèse de doctorat : Université de Fribourg, 2017 ; no. 2052.

Cette thèse de doctorat contient trois différents projets qui appartiennent aux domaines de la physique atomique des couches profondes et de la spectroscopie de rayons X en haute résolution. Le premier projet concerne l’étude des spectres d’absorption (XAS) K et L de quelques éléments de transition 3d, 4d et 5d. Les mesures ont été réalisées à Fribourg avec le spectromètre à...