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Université de Fribourg

Optical signature of a crossover from Mott- to Slater-type gap in ${\mathrm{Sr}}_{2}{\mathrm{Ir}}_{1\ensuremath{-}x}{\mathrm{Rh}}_{x}{\mathrm{O}}_{4}$

Xu, Bîng ; Marsik, Premysl ; Sheveleva, Evgeniia ; Lyzwa, Fryderyk ; Louat, A. ; Brouet, V. ; Munzar, Dominik ; Bernhard, Christian

In: Physical Review Letters, 2020, vol. 124, no. 2, p. 027402

With optical spectroscopy we provide evidence that the insulator-metal transition in Sr2Ir1−xRhxO4 occurs close to a crossover from the Mott- to the Slater-type. The Mott gap at x=0 persists to high temperature and evolves without an anomaly across the Néel temperature, TN. Upon Rh doping, it collapses rather rapidly and vanishes around x=0.055. Notably, just as the Mott gap vanishes yet...

Université de Fribourg

Growth and nanofabrication of all-perovskite superconducting/ferromagnetic/superconducting junctions

Andrés Prada, Roberto de ; Golod, T. ; Bernhard, Christian ; Krasnov, V. M.

In: Journal of Superconductivity and Novel Magnetism, 2019, vol. 32, no. 9, p. 2721–2726

We fabricate and study experimentally all-perovskite-oxide superconductor/ferromagnetic insulator/superconductor (S/FI/S) tunnel junctions made out of the high-temperature cuprate superconductor YBa2Cu3O7−y (YBCO) and the colossal magnetoresistive manganite LaMnO3 (LMO) in the ferromagnetic insulator state. YBCO/LMO/YBCO heterostructures with different LMO thicknesses (5, 10, and 20 nm)...

Université de Fribourg

Controlling the strength of ferromagnetic order in YBa2Cu3O7/La2/3Ca1/3MnO3 multilayers

Andrés Prada, Roberto de ; Gaina, Roxana ; Biškup, N. ; Varela, M. ; Stahn, J. ; Bernhard, Christian

In: Physical Review B, 2019, vol. 100, no. 11, p. 115129

With dc magnetization and polarized neutron reflectometry we studied the ferromagnetic response of YBa2Cu3O7/La2/3Ca1/3MnO3 (YBCO/LCMO) multilayers that are grown with pulsed laser deposition. We found that whereas for certain growth conditions (denoted as A type) the ferromagnetic moment of the LCMO layer is strongly dependent on the structural details of the YBCO layer on which it is ...

Université de Fribourg

Terahertz vortex beam as a spectroscopic probe of magnetic excitations

Sirenko, Andrei A. ; Maršík, Premysl ; Bernhard, Christian ; Stanislavchuk, T. N. ; Kiryukhin, V. ; Cheong, S.-W.

In: Physical Review Letters, 2019, vol. 122, no. 23, p. 237401

Circularly polarized light with spin angular momentum is one of the most valuable probes of magnetism. We demonstrate that light beams with orbital angular momentum (OAM), or vortex beams, can also couple to magnetism exhibiting dichroisms in a magnetized medium. Resonant optical absorption in a ferrimagnetic crystal depends strongly on both the handedness of the vortex and the direction of...

Université de Fribourg

Memory-functionality superconductor/ferromagnet/superconductor junctions based on the high- T c cuprate superconductors YBa 2 Cu 3 O 7 − x and the colossal magnetoresistive manganite ferromagnets La 2 / 3 X 1 / 3 MnO 3 + δ ( X = Ca , Sr )

Andrés Prada, R. de ; Golod, T. ; Kapran, O. M. ; Borodianskyi, E. A. ; Bernhard, Christian ; Krasnov, V. M.

In: Physical Review B, 2019, vol. 99, no. 21, p. 214510

Complex oxides exhibit a variety of unusual physical properties, which can be used for designing novel electronic devices. Here we fabricate and study experimentally nanoscale superconductor/ferromagnet/superconductor junctions with the high-Tc cuprate superconductors YBa2Cu3O7−x and the colossal magnetoresistive (CMR) manganite ferromagnets La2/3X1/3MnO3+δ (X=Ca or Sr). We demonstrate...

Université de Fribourg

Granular superconductivity and charge/orbital order in YBa 2 Cu 3 O 7 /manganite trilayers

Khmaladze, Jarji ; Sarkar, Subhrangsu ; Soulier, Mathias ; Lyzwa, Fryderyk ; Prada, R. de Andres ; Perret, Edith ; Mallett, Benjamin P. P. ; Minola, M. ; Keimer, B. ; Bernhard, Christian

In: Physical Review Materials, 2019, vol. 3, no. 8, p. 084801

We studied how the electronic, superconducting, and magnetic properties of YBa2Cu3O7/Nd1−x(Ca1−ySry )xMnO3 multilayers depend on the tolerance factor and the hole doping of the manganite. In particular, we investigated the granular superconducting state and the related magnetic-field-driven insulator-to- superconductor transition that was previously discovered in corresponding multilayers...

Université de Fribourg

Scaling of the Fano effect of the in-plane Fe-As phonon and the superconducting critical temperature in ${\mathrm{Ba}}_{1\ensuremath{-}x}{\mathrm{K}}_{x}{\mathrm{Fe}}_{2}{\mathrm{As}}_{2}$

Xu, Bing ; Cappelluti, E. ; Benfatto, Larra ; Mallett, Benjamin P. P. ; Marsik, Premysl ; Sheveleva, Evgeniia ; Lyzwa, Fryderyk ; Wolf, Thomas ; Yang, Rui ; Qiu, X. G. ; Dai, Y. M. ; Wen, H. H. ; Lobo, R. P. S. M. ; Bernhard, Christian

In: Physical Review Letters, 2019, vol. 122, no. 21, p. 217002

By means of infrared spectroscopy, we determine the temperature-doping phase diagram of the Fano effect for the in-plane Fe-As stretching mode in Ba1−xKxFe2As2. The Fano parameter 1=q2, which is a measure of the phonon coupling to the electronic particle-hole continuum, shows a remarkable sensitivity to the magnetic and structural orderings at low temperatures. Most strikingly, at elevated...

Université de Fribourg

Terahertz-driven phonon upconversion in SrTiO 3

Kozina, M. ; Fechner, M. ; Marsik, Premysl ; Driel, T. van ; Glownia, J. M. ; Bernhard, Christian ; Radovic, M. ; Zhu, D. ; Bonetti, S. ; Staub, U. ; Hoffmann, M. C.

In: Nature Physics, 2019, vol. 15, no. 4, p. 387–392

Direct manipulation of the atomic lattice using intense long-wavelength laser pulses has become a viable approach to create new states of matter in complex materials. Conventionally, a high-frequency vibrational mode is driven resonantly by a mid- infrared laser pulse and the lattice structure is modified through indirect coupling of this infrared-active phonon to other, lower-frequency...

Université de Fribourg

Signatures of the bonding-antibonding splitting in the $c$-axis infrared response of moderately underdoped bilayer and trilayer cuprate superconductors

Mallett, Benjamin P. P. ; Maršík, Premysl ; Munzar, Dominik ; Bernhard, Christian ; Dubroka, Adam

In: Physical Review B, 2019, vol. 99, no. 5, p. 054513

We report on results of our analysis of the c-axis infrared conductivity, σc(ω), of bilayer LnBa2Cu3O7−δ (Ln=La, Nd, Y) and trilayer Bi2Sr2Ca2Cu3O10+δ high-Tc superconductors. The analysis employs the multilayer model involving the conductivity of the bilayer or trilayer unit, σbl(ω), and that of the spacing layers separating the latter units, σint(ω). For the YBa2Cu3O7−δ sample...