Université de Fribourg

Superconductivity-induced transverse plasma mode and phonon anomaly in the $c$-axis response of the bilayer compound ${\mathrm{RbCa}}_{2}{\mathrm{Fe}}_{4}{\mathrm{As}}_{4}{\mathrm{F}}_{2}$

Xu, Bing ; Munzar, Dominik ; Dubroka, Adam ; Sheveleva, Evgeniia ; Lyzwa, Fryderyk ; Maršík, Premysl ; Wang, C. N. ; Wang, Z. C. ; Cao, G. H. ; Bernhard, Christian

In: Physical Review B, 2020, vol. 101, no. 21, p. 214512

We studied the infrared response of polycrystalline samples of the iron arsenide superconductor (Rb,Cs)Ca2Fe4As4F2 (Rb,Cs-12442), which has a bilayer structure similar to the high-Tc cuprates YBa2Cu3O7 (YBCO) and Bi2Sr2CaCu2O8. The c-axis reflectivity spectra Rc have been derived from the reflectivity spectra of the polycrystalline samples Rpoly and the in-plane spectrum of a corresponding...

Université de Fribourg

Signatures of the bonding-antibonding splitting in the $c$-axis infrared response of moderately underdoped bilayer and trilayer cuprate superconductors

Mallett, Benjamin P. P. ; Maršík, Premysl ; Munzar, Dominik ; Bernhard, Christian ; Dubroka, Adam

In: Physical Review B, 2019, vol. 99, no. 5, p. 054513

We report on results of our analysis of the c-axis infrared conductivity, σc(ω), of bilayer LnBa2Cu3O7−δ (Ln=La, Nd, Y) and trilayer Bi2Sr2Ca2Cu3O10+δ high-Tc superconductors. The analysis employs the multilayer model involving the conductivity of the bilayer or trilayer unit, σbl(ω), and that of the spacing layers separating the latter units, σint(ω). For the YBa2Cu3O7−δ sample...

Université de Fribourg

Infrared ellipsometry study of photogenerated charge carriers at the (001) and (110) surfaces of $\mathrm{SrTi}{\mathrm{O}}_{3}$ crystals and at the interface of the corresponding $\mathrm{LaAl}{\mathrm{O}}_{3}/\mathrm{SrTi}{\mathrm{O}}_{3}$ heterostructures

Yazdi-Rizi, Meghdad ; Maršík, Premysl ; Mallett, Benjamin P. P. ; Sen, Kaushik ; Cerreta, A. ; Dubroka, Adam ; Scigaj, M. ; Sánchez, F. ; Herranz, G. ; Bernhard, Christian

In: Physical Review B, 2017, vol. 95, no. 19, p. 195107

With infrared (IR) ellipsometry and dc resistance measurements, we investigated the photodoping at the (001) and (110) surfaces of SrTiO3 (STO) single crystals and at the corresponding interfaces of LaAlO3/SrTiO3 (LAO/STO) heterostructures. In the bare STO crystals, we find that the photogenerated charge carriers, which accumulate near the (001) surface, have a similar depth profile and sheet...

Université de Fribourg

Infrared ellipsometry study of the confined electrons in a high-mobility γ-Al₂O₃/SrTiO₃ heterostructure

Yazdi-Rizi, Meghdad ; Maršík, Premysl ; Mallett, Benjamin P. P. ; Dubroka, Adam ; Christensen, D. V. ; Chen, Y. Z. ; Pryds, N. ; Bernhard, Christian

In: EPL (Europhysics Letters), 2016, vol. 113, no. 4, p. 47005

With infrared ellipsometry we studied the response of the confined electrons in γ-Al₂O₃/SrTiO₃ (GAO/STO) heterostructures in which they originate predominantly from oxygen vacancies. From the analysis of a so-called Berreman mode, that develops near the highest longitudinal optical phonon mode of SrTiO₃, we derive the sheet carrier density, N s , the...

Université de Fribourg

Evidence for precursor superconducting pairing above T c in underdoped cuprates from an analysis of the in-plane infrared response

Šopík, B. ; Chaloupka, Jiří ; Dubroka, Adam ; Bernhard, Christian ; Munzar, Dominik

In: New Journal of Physics, 2015, vol. 17, no. 5, p. 053022

We performed calculations of the in-plane infrared response of underdoped cuprate superconductors to clarify the origin of a characteristic dip feature which occurs in the published experimental spectra of the real part of the in-plane conductivity below an onset temperature ${{T}^{{\rm ons}}}$ considerably higher than ${{T}_{{\rm c}}}$. We provide several arguments, based on a detailed...

Université de Fribourg

Low-energy interband transitions in the infrared response of Ba(Fe1-xCox)2As2

Maršík, Premysl ; Wang, Chen Nan ; Rössle, Matthias ; Yazdi-Rizi, M. ; Schuster, Roman ; Kim, Kyung Wan ; Dubroka, Adam ; Munzar, Dominik ; Wolf, T. ; Chen, X. H. ; Bernhard, Christian

In: Physical Review B, 2014, vol. 88, no. 18, p. 180508

We studied the doping and temperature (T) dependence of the infrared (IR) response of Ba(Fe1−xCox)2As2 single crystals. We show that a weak band around 1000 cm−1, that was previously interpreted in terms of interaction of the charge carriers with magnetic excitations or of a pseudogap, is rather related to low-energy interband transitions. Specifically, we show that this band exhibits a...

Université de Fribourg

Optical probe of ferroelectric order in bulk and thin-film perovskite titanates

Rössle, Matthias ; Wang, Chen Nan ; Maršík, Premysl ; Yazdi-Rizi, M. ; Kim, Kyung Wan ; Dubroka, Adam ; Marozau, Ivan ; Schneider, C. W. ; Humlíček, J. ; Baeriswyl, Dionys ; Bernhard, Christian

In: Physical Review B, 2013, vol. 88, no. 10, p. 104110

We have measured the temperature dependence of the direct band gap Eg in SrTiO₃ and BaTiO₃ and related materials with quantum-paraelectric and ferroelectric properties using optical spectroscopy. We show that Eg exhibits an anomalous temperature dependence with pronounced changes in the vicinity of the ferroelectric transition that can be...

Université de Fribourg

Electric-Field-Induced Polar Order and Localization of the Confined Electrons in LaAlO₃/SrTiO₃ Heterostructures

Rössle, Matthias ; Kim, Kyung Wan ; Dubroka, Adam ; Maršík, Premysl ; Wang, Chen Nan ; Jany, R. ; Richter, C. ; Mannhart, J. ; Schneider, C. W. ; Frano, A. ; Wochner, P. ; Lu, Y. ; Keimer, B. ; Shukla, D. K. ; Strempfer, J. ; Bernhard, Christian

In: Physical Review Letters, 2013, vol. 110, no. 13, p. 136805

With ellipsometry, x-ray diffraction, and resistance measurements we investigated the electric-field effect on the confined electrons at the LaAlO₃/SrTiO₃ interface. We obtained evidence that the localization of the electrons at negative gate voltage is induced, or at least enhanced, by a polar phase transition in SrTiO₃ which strongly reduces the lattice polarizability and the subsequent...

Université de Fribourg

Far-infrared spectra of the magnetic exchange resonances and optical phonons and their connection to magnetic and dielectric properties of Dy₃Fe₅O₁₂ garnet

Kang, T. D. ; Standard, E. C. ; Rogers, P. D. ; Ahn, K. H. ; Sirenko, Andrei A. ; Dubroka, Adam ; Bernhard, Christian ; Park, S. ; Choi, Y. J. ; Cheong, S.-W.

In: Physical Review B - Condensed Matter and Materials Physics, 2012, vol. 86, no. 14, p. 144112

Far-infrared spectra of ferrimagnetic Dy₃Fe₅O₁₂ single crystals have been studied in the spectral range between 12 and 700 cm⁻¹ and in a wide temperature range between 5 K and 300 K using transmission spectroscopy and rotating analyzer ellipsometry. In the temperature range below TC = 16 K for the magnetic ordering of Dy³⁺ spins, a number of ligand field and...

Université de Fribourg

Macroscopic phase segregation in superconducting K0.73Fe1.67Se₂ as seen by muon spin rotation and infrared spectroscopy

Wang, Chen Nan ; Maršik, Premysl ; Schuster, Roman ; Dubroka, Adam ; Rössle, Matthias ; Niedermayer, Ch. ; Varma, G. D. ; Wang, A. F. ; Chen, X. H. ; Wolf, T. ; Bernhard, Christian

In: Physical Review B - Condensed matter and materials physics, 2012, vol. 85, no. 21, p. 214503

Using muon spin rotation and infrared spectroscopy, we investigated the recently discovered superconductor K0.73Fe1.67Se₂ with Tc≈32 K. We show that the combined data can be consistently described in terms of a macroscopically phase-segregated state with a matrix of ∼88% volume fraction that is insulating and strongly magnetic and inclusions with an ∼12%...