Université de Fribourg

Muon spin rotation and infrared spectroscopy study of Ba$_{1-x}$Na$_{x}$Fe$_{2}$As$_{2}$

Sheveleva, Evgeniia ; Xu, Bing ; Marsik, Premysl ; Lyzwa, Fryderyk ; Mallett, Benjamin P. P. ; Willa, K. ; Meingast, C. ; Wolf, Th. ; Shevtsova, T. ; Pashkevich, Yu. G. ; Bernhard, Christian

In: Physical Review B, 2020, vol. 101, no. 22, p. 224515

The magnetic and superconducting properties of a series of underdoped Ba 1 − x Na x Fe 2 As 2 (BNFA) single crystals with 0.19 ≤ x ≤ 0.34 have been investigated with the complementary muon-spin-rotation ( μ SR ) and infrared spectroscopy techniques. The focus has been on the different antiferromagnetic states in the underdoped regime and their competition with superconductivity,...

Université de Fribourg

Backfolded acoustic phonons as ultrasonic probes in metal-oxide superlattices

Lyzwa, Fryderyk ; Chan, A. ; Khmaladze, Jarji ; Fürsich, K. ; Keimer, B. ; Bernhard, Christian ; Minola, M. ; Mallett, Benjamin P. P.

In: Physical Review Materials, 2020, vol. 4, no. 4, p. 043606

Ultrasonics have been an incisive probe of internal interfaces in a wide variety of systems ranging from stars to solids. For thin-film structures, however, ultrasound is largely ineffective because the signal is dominated by the substrate. Using confocal Raman spectromicroscopy, we show that multiple reflection of sound waves at internal interfaces of a metal-oxide superlattice generates...

Université de Fribourg

Granular superconductivity and charge/orbital order in YBa 2 Cu 3 O 7 /manganite trilayers

Khmaladze, Jarji ; Sarkar, Subhrangsu ; Soulier, Mathias ; Lyzwa, Fryderyk ; Prada, R. de Andres ; Perret, Edith ; Mallett, Benjamin P. P. ; Minola, M. ; Keimer, B. ; Bernhard, Christian

In: Physical Review Materials, 2019, vol. 3, no. 8, p. 084801

We studied how the electronic, superconducting, and magnetic properties of YBa2Cu3O7/Nd1−x(Ca1−ySry )xMnO3 multilayers depend on the tolerance factor and the hole doping of the manganite. In particular, we investigated the granular superconducting state and the related magnetic-field-driven insulator-to- superconductor transition that was previously discovered in corresponding multilayers...

Université de Fribourg

Scaling of the Fano effect of the in-plane Fe-As phonon and the superconducting critical temperature in ${\mathrm{Ba}}_{1\ensuremath{-}x}{\mathrm{K}}_{x}{\mathrm{Fe}}_{2}{\mathrm{As}}_{2}$

Xu, Bing ; Cappelluti, E. ; Benfatto, Larra ; Mallett, Benjamin P. P. ; Marsik, Premysl ; Sheveleva, Evgeniia ; Lyzwa, Fryderyk ; Wolf, Thomas ; Yang, Rui ; Qiu, X. G. ; Dai, Y. M. ; Wen, H. H. ; Lobo, R. P. S. M. ; Bernhard, Christian

In: Physical Review Letters, 2019, vol. 122, no. 21, p. 217002

By means of infrared spectroscopy, we determine the temperature-doping phase diagram of the Fano effect for the in-plane Fe-As stretching mode in Ba1−xKxFe2As2. The Fano parameter 1=q2, which is a measure of the phonon coupling to the electronic particle-hole continuum, shows a remarkable sensitivity to the magnetic and structural orderings at low temperatures. Most strikingly, at elevated...

Université de Fribourg

Signatures of the bonding-antibonding splitting in the $c$-axis infrared response of moderately underdoped bilayer and trilayer cuprate superconductors

Mallett, Benjamin P. P. ; Maršík, Premysl ; Munzar, Dominik ; Bernhard, Christian ; Dubroka, Adam

In: Physical Review B, 2019, vol. 99, no. 5, p. 054513

We report on results of our analysis of the c-axis infrared conductivity, σc(ω), of bilayer LnBa2Cu3O7−δ (Ln=La, Nd, Y) and trilayer Bi2Sr2Ca2Cu3O10+δ high-Tc superconductors. The analysis employs the multilayer model involving the conductivity of the bilayer or trilayer unit, σbl(ω), and that of the spacing layers separating the latter units, σint(ω). For the YBa2Cu3O7−δ sample...

Université de Fribourg

Lattice-mediated magnetic order melting in ${\mathrm{TbMnO}}_{3}$

Baldini, Edoardo ; Kubacka, Teresa ; Mallett, Benjamin P. P. ; Ma, Chao ; Koohpayeh, Seyed M. ; Zhu, Yimei ; Bernhard, Christian ; Johnson, Steven L. ; Carbone, Fabrizio

In: Physical Review B, 2018, vol. 97, no. 12, p. 125149

Recent ultrafast magnetic-sensitive measurements [Johnson et al., Phys. Rev. B 92, 184429 (2015); Bothschafter et al., Phys. Rev. B 96, 184414 (2017)] have revealed a delayed melting of the long-range cycloid spin order in TbMnO3 following photoexcitation across the fundamental Mott-Hubbard gap. The microscopic mechanism behind this slow transfer of energy from the photoexcited carriers to...

Université de Fribourg

Structural, magnetic and electronic properties of pulsed-laser-deposition grown SrFeO 3− δ thin films and SrFeO 3− δ /La 2/3 Ca 1/3 MnO 3 multilayers

Perret, Edith ; Sen, Kaushik ; Khmaladze, Jarji ; Mallett, Benjamin P. P. ; Yazdi-Rizi, Meghdad ; Maršík, Premysl ; Das, Saikat ; Marozau, Ivan ; Uribe-Laverde, Miguel Angel ; Andrés Prada, R. de ; Strempfer, J. ; Döbeli, Max ; Biškup, N. ; Varela, M. ; Mathis, Y.-L. ; Bernhard, Christian

In: Journal of Physics: Condensed Matter, 2017, vol. 29, no. 49, p. 495601

We studied the structural, magnetic and electronic properties of ${\rm SrFeO}_{3- \delta}$ (SFO) thin films and ${\rm SrFeO}_{3-\delta}$ /${\rm La}_{2/3}$ ${\rm Ca}_{1/3}$ MnO3 (LCMO) superlattices that have been grown with pulsed laser deposition (PLD) on ${\rm La}_{0.3}$ ${\rm Sr}_{0.7}$ ${\rm Al}_{0.65}$ ${\rm Ta}_{0.35}$ ${\rm O}_{3}$ (LSAT) substrates. X-ray reflectometry and scanning ...

Université de Fribourg

Infrared ellipsometry study of photogenerated charge carriers at the (001) and (110) surfaces of $\mathrm{SrTi}{\mathrm{O}}_{3}$ crystals and at the interface of the corresponding $\mathrm{LaAl}{\mathrm{O}}_{3}/\mathrm{SrTi}{\mathrm{O}}_{3}$ heterostructures

Yazdi-Rizi, Meghdad ; Maršík, Premysl ; Mallett, Benjamin P. P. ; Sen, Kaushik ; Cerreta, A. ; Dubroka, Adam ; Scigaj, M. ; Sánchez, F. ; Herranz, G. ; Bernhard, Christian

In: Physical Review B, 2017, vol. 95, no. 19, p. 195107

With infrared (IR) ellipsometry and dc resistance measurements, we investigated the photodoping at the (001) and (110) surfaces of SrTiO3 (STO) single crystals and at the corresponding interfaces of LaAlO3/SrTiO3 (LAO/STO) heterostructures. In the bare STO crystals, we find that the photogenerated charge carriers, which accumulate near the (001) surface, have a similar depth profile and sheet...

Université de Fribourg

Strongly bound excitons in anatase TiO₂ single crystals and nanoparticles

Baldini, Eduardo ; Chiodo, Letizia ; Dominguez, A. ; Palummo, M. ; Moser, S. ; Yazdi-Rizi, Meghdad ; Auböck, G. ; Mallett, Benjamin P. P. ; Berger, Helmuth ; Magrez, Arnaud ; Bernhard, Christian ; Grioni, M. ; Rubio, Angel ; Chergui, Majed

In: Nature Communications, 2017, vol. 8, no. 1, p. 13

Anatase TiO₂ is among the most studied materials for light-energy conversion applications, but the nature of its fundamental charge excitations is still unknown. Yet it is crucial to establish whether light absorption creates uncorrelated electron–hole pairs or bound excitons and, in the latter case, to determine their character. Here, by combining steady-state angle-resolved...

Université de Fribourg

Muon spin rotation and infrared spectroscopy study of magnetism and superconductivity in ${\mathrm{Ba}}_{1\ensuremath{-}x}{\mathrm{K}}_{x}{\mathrm{Fe}}_{2}{\mathrm{As}}_{2}$

Mallett, Benjamin P. P. ; Wang, Chen Nan ; Marsik, Premysl ; Sheveleva, Evgeniia ; Yazdi-Rizi, Meghdad ; Tallon, Jeffery L. ; Adelmann, P. ; Wolf, Th. ; Bernhard, Christian

In: Physical Review B, 2017, vol. 95, no. 5, p. 054512

Using muon spin rotation and infrared spectroscopy, we study the relation between magnetism and superconductivity in Ba1−xKxFe2As2 single crystals from the underdoped to the slightly overdoped regime. We find that the Fe magnetic moment is only moderately suppressed in most of the underdoped region where it decreases more slowly than the Néel temperature TN. This applies for both the total...