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Université de Fribourg

Strain-induced ferromagnetism in antiferromagnetic LuMnO₃ thin films

White, J. S. ; Bator, M. ; Hu, Yanqing ; Luetkens, H. ; Stahn, J. ; Capelli, S. ; Das, Saikat ; Döbeli, M. ; Lippert, Th. ; Malik, Vivek Kumar ; Martynczuk, J. ; Wokaun, A. ; Kenzelmann, M. ; Niedermayer, Ch. ; Schneider, C. W.

In: Physical Review Letters, 2013, vol. 111, no. 3, p. 037201

Single phase and strained LuMnO₃ thin films are discovered to display coexisting ferromagnetic and antiferromagnetic orders. A large moment ferromagnetism (≈1μB), which is absent in bulk samples, is shown to display a magnetic moment distribution that is peaked at the highly strained substrate-film interface. We further show that the strain-induced ferromagnetism and the...

Université de Fribourg

Depth profile of the ferromagnetic order in a YBa₂Cu₃O₇/La2/3Ca1/3MnO₃ superlattice on a LSAT substrate: A polarized neutron reflectometry study

Uribe-Laverde, Miguel Angel ; Satapathy, Dillip Kumar ; Marozau, Ivan ; Malik, Vivek Kumar ; Das, Saikat ; Sen, Kaushik ; Stahn, J. ; Rühm, A. ; Kim, Joo Young ; Keller, T. ; Devishvili, A. ; Toperverg, B. P. ; Bernhard, Christian

In: Physical Review B - Condensed Matter and Materials Physics, 2013, vol. 87, no. 11, p. 115105

Using polarized neutron reflectometry (PNR) we have investigated a [YBa₂Cu₃O₇(10 nm)/La2/3Ca1/3MnO₃(9 nm)]₁₀ (YBCO/LCMO) superlattice grown by pulsed laser deposition on a La0.3Sr0.7Al0.65Ta0.35O₃ (LSAT) substrate. Due to the high structural quality of the superlattice and the substrate, the specular reflectivity...

Université de Fribourg

Spatially resolved strain-imprinted magnetic states in an artificial multiferroic

Chopdekar, R. V. ; Malik, Vivek Kumar ; Rodríguez, A. Fraile ; Guyader, L. Le ; Takamura, Y. ; Scholl, A. ; Stender, D. ; Schneider, C. W. ; Bernhard, Christian ; Nolting, F. ; Heyderman, L. J.

In: Physical Review B - Condensed Matter and Materials Physics, 2012, vol. 86, no. 01, p. 014408

Artificial multiferroic systems, in which novel properties can emerge from elastic coupling between piezoelectric and magnetostrictive phases, are a promising route to obtain significant room-temperature magnetoelectric coupling at the nanoscale. In this work, we have used element-specific soft x-ray photoemission electron microscopy to spatially resolve the effects of ferroelectric BaTiO₃ on...

Université de Fribourg

Magnetic Proximity Effect in YBa₂Cu₃O₇/La2/3Ca1/3MnO₃ and YBa₂Cu₃O₇/LaMnO₃₊ Superlattices

Satapathy, Dillip Kumar ; Uribe-Laverde, M. A. ; Marozau, I. ; Malik, Vivek K. ; Das, S. ; Wagner, Th. ; Marcelot, C. ; Stahn, J. ; Brück, S. ; Rühm, A. ; Macke, S. ; Tietze, T. ; Goering, E. ; Frañó, A. ; Kim, J. -H. ; Wu, M. ; Benckiser, E. ; Keimer, B. ; Devishvili, A. ; Toperverg, B. P. ; Merz, M. ; Nagel, P. ; Schuppler, S. ; Bernhard, Christian

In: Physical Review Letters, 2012, vol. 108, no. 19, p. 197201

Using neutron reflectometry and resonant x-ray techniques we studied the magnetic proximity effect (MPE) in superlattices composed of superconducting YBa₂Cu₃O₇ and ferromagnetic-metallic La0.67Ca0.33MnO₃ or ferromagnetic-insulating LaMnO₃₊. We find that the MPE strongly depends on the electronic state of the manganite layers, being pronounced for the...

Université de Fribourg

Pulsed laser deposition growth of heteroepitaxial YBa2Cu3O7/La0.67Ca0.33MnO3 superlattices on NdGaO3 and Sr0.7La0.3Al0.65Ta0.35O3 substrates

Malik, Vivek Kumar ; Marozau, I. ; Das, S. ; Doggett, B. ; Satapathy, Dillip Kumar ; Uribe-Laverde, M. A. ; Biskup, N. ; Varela, M. ; Schneider, C. W. ; Marcelot, C. ; Stahn, J. ; Bernhard, Christian

In: Physical Review B - Condensed matter and materials physics, 2012, vol. 85, no. 5, p. 054514

Heteroepitaxial superlattices of [YBa₂Cu₃O₇(n)/La0.67Ca0.33MnO₃(m)]x (YBCO/LCMO), where n and m are the number of YBCO and LCMO monolayers and x the number of bilayer repetitions, have been grown with pulsed laser deposition on NdGaO₃ (110) and Sr0.7La0.3Al0.65Ta0.35O₃ (001). These substrates are well lattice...

Université de Fribourg

Magnetism, superconductivity, and coupling in cuprate heterostructures probed by low-energy muon-spin rotation

Wojek, B. M. ; Morenzoni, E. ; Eshchenko, D. G. ; Suter, A. ; Prokscha, T. ; Keller, H. ; Koller, E. ; Fischer, Ø. ; Malik, Vivek Kumar ; Bernhard, Christian ; Döbeli, M.

In: Physical Review B - Condensed matter and materials physics, 2012, vol. 85, no. 2, p. 024505

We present a low-energy muon-spin-rotation study of the magnetic and superconducting properties of YBa₂Cu₃O7−δ/PrBa₂Cu₃O7−δ trilayer and bilayer heterostructures. By determining the magnetic-field profiles throughout these structures, we show that a finite superfluid density can be induced in otherwise semiconducting PrBa₂Cu₃O7−δ layers...

Université de Fribourg

DC magnetization investigations in Ti1−xMnxO₂ nanocrystalline powder

Sharma, Sudesh ; Chaudhary, Sujeet ; Kashyap, Subhash C. ; Malik, Vivek K.

In: Journal of Alloys and Compounds, 2011, vol. 509, no. 27, p. 7434-7438

In the present paper, DC magnetization investigation on the insulating nanocrystalline powder samples of Ti1−xMnxO₂ (x = 0, 0.05, 0.10, and 0.15) prepared by simple chemical route is reported. Structural measurements revealed phase pure anatase structure of TiO₂ when x ≤ 0.05 and a mixture of anatase and rutile TiO₂ along with the...

Université de Fribourg

Dimensionality control of electronic phase transitions in nickel-Oxide superlattices

Boris, A. V. ; Matiks, Y. ; Benckiser, E. ; Frano, A. ; Popovich, P. ; Hinkov, V. ; Wochner, P. ; Castro-Colin, M. ; Detemple, E. ; Malik, Vivek Kumar ; Bernhard, Christian ; Prokscha, T. ; Suter, A. ; Salman, Z. ; Morenzoni, E. ; Cristiani, G. ; Habermeier, H.-U. ; Keimer, B.

In: Science, 2011, vol. 332, no. 6032, p. 937-940

The competition between collective quantum phases in materials with strongly correlated electrons depends sensitively on the dimensionality of the electron system, which is difficult to control by standard solid-state chemistry. We have fabricated superlattices of the paramagnetic metal lanthanum nickelate (LaNiO₃) and the wide-gap insulator lanthanum aluminate (LaAlO₃) with atomically...

Université de Fribourg

Engineering spin propagation across a hybrid organic/inorganic interface using a polar layer

Schulz, Leander ; Nuccio, L. ; Willis, M. ; Desai, P. ; Shakya, P. ; Kreouzis, T. ; Malik, Vivek Kumar ; Bernhard, Christian ; Pratt, F. L. ; Morley, N. A. ; Suter, A. ; Nieuwenhuys, G. J. ; Prokscha, T. ; Morenzoni, E. ; Gillin, W. P. ; Drew, Alan J.

In: Nature Materials, 2011, vol. 10, p. 39–44

Spintronics has shown a remarkable and rapid development, for example from the initial discovery of giant magnetoresistance in spin valves (Baibich, M. N. et al. Giant magnetoresistance of (001)Fe/(001)Cr magnetic superlattices. Phys. Rev. Lett. 61, 2472–2475, 1988) to their ubiquity in hard-disk read heads in a relatively short time. However, the ability to fully harness electron spin as...