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    Université de Fribourg

    Effect of charge order on the plasmon dispersion in transition-metal dichalcogenides

    Wezel, Jasper van ; Schuster, Roman ; König, Andreas ; Knupfer, Martin ; Brink, Jeroen van den ; Berger, Helmuth ; Büchner, Bernd

    In: Physical Review Letters, 2011, vol. 107, no. 17, p. 176404

    We investigate the dispersion of the charge carrier plasmon in the three prototypical charge-density wave bearing transition-metal dichalcogenides 2H-TaSe₂, 2H-TaS₂, and 2H-NbSe₂ employing electron energy-loss spectroscopy. For all three compounds the plasmon dispersion is found to be negative for small momentum transfers. This is in contrast with the generic behavior observed in simple...