In: Physical Review A, 2014, vol. 88, no. 5, p. 052505
A detailed investigation of the Lα1,2 (L3→M4,5) and Lβ1 (L2→M4) x-ray satellite and hypersatellite structures in zirconium, molybdenum, and palladium atoms multiply ionized by impact with 278.6-MeV oxygen ions is reported. The x-ray spectra were measured with a high-resolution von Hamos bent crystal spectrometer. For the interpretation of the complex spectral features, relativistic...
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In: Physical Review A, 2014, vol. 88, no. 5, p. 052506
We report on high-resolution measurements of the photoinduced L1M2 and L1M3 x-ray emission lines of 69Tm, 70Yb, 71Lu, 73Ta, 74W, 75Re, 77Ir, 81Tl, 83Bi, and 95Am. From the linewidths of the measured transitions an accurate set of M2 and M3 level widths is determined assuming for the L1 level widths the values reported by Raboud [P.-A. Raboud et al., Phys. Rev. A 65, 022512 (2002)]. Furthermore,...
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In: Review of Scientific Instruments, 2013, vol. 84, no. 9, p. 093104
We report on a high-resolution transmission-type curved crystal spectrometer based on the modified DuMond slit geometry. The spectrometer was developed at the University of Fribourg for the study of photoinduced X-ray spectra. K and L X-ray transitions with energies above about 10 keV can be measured with an instrumental resolution comparable to their natural linewidths. Construction details...
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In: Journal of Analytical Atomic Spectrometry, 2013, vol. 28, no. 5, p. 689–696
X-ray Standing Wave (XSW) is a well established formalism for modelling Grazing Incidence X-ray Fluorescence (GIXRF) experiments. However, when probing nanostructured surfaces with complex morphology the effects of the interaction of the XSW with structure elements need to be investigated. This is not always easy and sometimes even not possible. In the present work a novel approach employing...
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In: Journal of Physics: Conference Series, 2012, vol. 388, no. 6, p. 062044
Observed enhancement of K-shell radiative recombination (RR) of bare uranium ions with cooling electrons is interpreted in terms of of distant transverse collisions in magnetized electron-cooler plasma described within the semiclassical geometrical model (SGM), which was recently proposed. The Monte Carlo simulations based on the proposed approach explains the enhancement measured in RR of...
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In: Review of Scientific Instruments, 2012, vol. 83, no. 10, p. 103105
We report on the design and performance of a wavelength-dispersive type spectrometer based on the von Hamos geometry. The spectrometer is equipped with a segmented-type crystal for x-ray diffraction and provides an energy resolution in the order of 0.25 eV and 1 eV over an energy range of 8000 eV–9600 eV. The use of a segmented crystal results in a simple and straightforward crystal...
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In: Journal of Electron Spectroscopy and Related Phenomena, 2012, p. -
The mechanisms leading to the production of hollow K shell atoms via single photon impact were investigated for a variety of light elements with 12 ≤ Z ≤ 23. The double 1s vacancy states were produced by irradiating the samples with intense monoenergetic synchrotron radiation beams. The double-to-single K-shell photoionization probabilities...
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In: X-Ray Spectrometry, 2012, vol. 41, no. 2, p. 98-104
We report on the surface-sensitive grazing emission X-ray fluorescence technique combined with synchrotron radiation excitation and high-resolution detection to realize depth-profile measurements of Al-implanted Si wafers. The principles of grazing emission measurements as well as the benefits offered by synchrotron sources and wavelength-dispersive detection setups are presented. It is shown...
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In: Physical Review Letters, 2011, vol. 107, no. 7, p. 073001
We propose a novel approach for the theoretical analysis of the photoinduced high-resolution Khα1,2 x-ray hypersatellite spectra, which allows us to obtain reliable values of lifetimes of the doubly K-shell ionized states and fundamental information about the relative role of K-shell double photoionization (DPI) mechanisms. It is demonstrated for the first time that the...
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In: Physical Review Letters, 2011, vol. 107, no. 5, p. 053001
xperimental evidence for the correlated two-electron one-photon transitions (1s⁻²→2s⁻¹2p⁻¹) following single-photon K-shell double ionization is reported. The double K-shell vacancy states in solid Mg, Al, and Si were produced by means of monochromatized synchrotron radiation, and the two-electron one-photon radiative transitions were observed by using a wavelength dispersive...
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