Université de Fribourg

Spatially resolved strain-imprinted magnetic states in an artificial multiferroic

Chopdekar, R. V. ; Malik, Vivek Kumar ; Rodríguez, A. Fraile ; Guyader, L. Le ; Takamura, Y. ; Scholl, A. ; Stender, D. ; Schneider, C. W. ; Bernhard, Christian ; Nolting, F. ; Heyderman, L. J.

In: Physical Review B - Condensed Matter and Materials Physics, 2012, vol. 86, no. 01, p. 014408

Artificial multiferroic systems, in which novel properties can emerge from elastic coupling between piezoelectric and magnetostrictive phases, are a promising route to obtain significant room-temperature magnetoelectric coupling at the nanoscale. In this work, we have used element-specific soft x-ray photoemission electron microscopy to spatially resolve the effects of ferroelectric BaTiO₃ on...

Université de Fribourg

Structural, magnetic, and superconducting properties of pulsed-laser-deposition-grown ${\text{La}}_{1.85}$${\text{Sr}}_{0.15}$${\text{CuO}}_{4}$/${\text{La}}_{2/3}$${\text{Ca}}_{1/3}$${\text{MnO}}_{3}$ superlattices on (001)-oriented ${\text{LaSrAlO}}_{4}$ substrates

Das, Saikat ; Sen, Kaushik ; Marozau, Ivan ; Uribe-Laverde, Miguel Angel ; Biskup, N. ; Varela, M. ; Khaydukov, Y. ; Soltwedel, O. ; Keller, T. ; Döbeli, M. ; Schneider, C. W. ; Bernhard, Christian

In: Physical Review B, 2014, vol. 89, no. 9, p. 094511

Epitaxial La1.85Sr0.15CuO4/La2/3Ca1/3MnO3 (LSCO/LCMO) superlattices on (001)-oriented LaSrAlO4 substrates have been grown with pulsed laser deposition technique. Their structural, magnetic, and superconducting properties have been determined with in situ reflection high-energy electron diffraction, x-ray diffraction, specular neutron reflectometry, scanning transmission electron microscopy,...

Université de Fribourg

Dynamical response and confinement of the electrons at the LaAlO₃/SrTiO₃ interface

Dubroka, Adam ; Rössle, Matthias ; Kim, Kyung Wan ; Malik, Vivek Kumar ; Schulz, Leander ; Thiel, S. ; Schneider, C. W. ; Mannhart, J. ; Herranz, G. ; Copie, O. ; Bibes, M. ; Barthélémy, A. ; Bernhard, Christian

In: Physical Review Letters, 2010, vol. 104, p. 156807

With infrared ellipsometry and transport measurements we investigated the electrons at the interface between LaAlO₃ and SrTiO₃. We obtained a sheet carrier concentration of Ns≈5–9×10¹³ cm⁻², an effective mass of m*=3.2±0.4me, and a strongly frequency dependent mobility. The latter are similar as in bulk SrTi1-xNbxO₃ and...

Université de Fribourg

Pulsed laser deposition growth of heteroepitaxial YBa2Cu3O7/La0.67Ca0.33MnO3 superlattices on NdGaO3 and Sr0.7La0.3Al0.65Ta0.35O3 substrates

Malik, Vivek Kumar ; Marozau, I. ; Das, S. ; Doggett, B. ; Satapathy, Dillip Kumar ; Uribe-Laverde, M. A. ; Biskup, N. ; Varela, M. ; Schneider, C. W. ; Marcelot, C. ; Stahn, J. ; Bernhard, Christian

In: Physical Review B - Condensed matter and materials physics, 2012, vol. 85, no. 5, p. 054514

Heteroepitaxial superlattices of [YBa₂Cu₃O₇(n)/La0.67Ca0.33MnO₃(m)]x (YBCO/LCMO), where n and m are the number of YBCO and LCMO monolayers and x the number of bilayer repetitions, have been grown with pulsed laser deposition on NdGaO₃ (110) and Sr0.7La0.3Al0.65Ta0.35O₃ (001). These substrates are well lattice...

Université de Fribourg

Optical probe of ferroelectric order in bulk and thin-film perovskite titanates

Rössle, Matthias ; Wang, Chen Nan ; Maršík, Premysl ; Yazdi-Rizi, M. ; Kim, Kyung Wan ; Dubroka, Adam ; Marozau, Ivan ; Schneider, C. W. ; Humlíček, J. ; Baeriswyl, Dionys ; Bernhard, Christian

In: Physical Review B, 2013, vol. 88, no. 10, p. 104110

We have measured the temperature dependence of the direct band gap Eg in SrTiO₃ and BaTiO₃ and related materials with quantum-paraelectric and ferroelectric properties using optical spectroscopy. We show that Eg exhibits an anomalous temperature dependence with pronounced changes in the vicinity of the ferroelectric transition that can be...

Université de Fribourg

Electric-Field-Induced Polar Order and Localization of the Confined Electrons in LaAlO₃/SrTiO₃ Heterostructures

Rössle, Matthias ; Kim, Kyung Wan ; Dubroka, Adam ; Maršík, Premysl ; Wang, Chen Nan ; Jany, R. ; Richter, C. ; Mannhart, J. ; Schneider, C. W. ; Frano, A. ; Wochner, P. ; Lu, Y. ; Keimer, B. ; Shukla, D. K. ; Strempfer, J. ; Bernhard, Christian

In: Physical Review Letters, 2013, vol. 110, no. 13, p. 136805

With ellipsometry, x-ray diffraction, and resistance measurements we investigated the electric-field effect on the confined electrons at the LaAlO₃/SrTiO₃ interface. We obtained evidence that the localization of the electrons at negative gate voltage is induced, or at least enhanced, by a polar phase transition in SrTiO₃ which strongly reduces the lattice polarizability and the subsequent...

Université de Fribourg

Strain-induced ferromagnetism in antiferromagnetic LuMnO₃ thin films

White, J. S. ; Bator, M. ; Hu, Yanqing ; Luetkens, H. ; Stahn, J. ; Capelli, S. ; Das, Saikat ; Döbeli, M. ; Lippert, Th. ; Malik, Vivek Kumar ; Martynczuk, J. ; Wokaun, A. ; Kenzelmann, M. ; Niedermayer, Ch. ; Schneider, C. W.

In: Physical Review Letters, 2013, vol. 111, no. 3, p. 037201

Single phase and strained LuMnO₃ thin films are discovered to display coexisting ferromagnetic and antiferromagnetic orders. A large moment ferromagnetism (≈1μB), which is absent in bulk samples, is shown to display a magnetic moment distribution that is peaked at the highly strained substrate-film interface. We further show that the strain-induced ferromagnetism and the...