In: Nature Communications, 2020, vol. 11, no. 1, p. 850
In a seminal paper, Mahan predicted that excitonic bound states can still exist in a semiconductor at electron-hole densities above the insulator-to-metal Mott transition. However, no clear evidence for this exotic quasiparticle, dubbed Mahan exciton, exists to date at room temperature. In this work, we combine ultrafast broadband optical spectroscopy and advanced many-body calculations to...
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In: Proceedings of the National Academy of Sciences, 2020, vol. 117, no. 12, p. 6409-6416
The role of the crystal lattice for the electronic properties of cuprates and other high-temperature superconductors remains controversial despite decades of theoretical and experimental efforts. While the paradigm of strong electronic correlations suggests a purely electronic mechanism behind the insulator-to-metal transition, recently the mutual enhancement of the electron–electron and the...
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In: Physical Review B, 2018, vol. 97, no. 12, p. 125149
Recent ultrafast magnetic-sensitive measurements [Johnson et al., Phys. Rev. B 92, 184429 (2015); Bothschafter et al., Phys. Rev. B 96, 184414 (2017)] have revealed a delayed melting of the long-range cycloid spin order in TbMnO3 following photoexcitation across the fundamental Mott-Hubbard gap. The microscopic mechanism behind this slow transfer of energy from the photoexcited carriers to...
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In: Physical Review B, 2017, vol. 96, no. 4, p. 041204
Elucidating the details of electron-phonon coupling in semiconductors and insulators is a topic of pivotal interest, as it governs the transport mechanisms and is responsible for various phenomena such as spectral-weight transfers to phonon sidebands and self-trapping. Here, we investigate the influence of the electron-phonon interaction on the excitonic peaks of rutile TiO2, revealing a strong...
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In: Physical Review B, 2017, vol. 95, no. 2, p. 024501
In cuprates, a precursor state of superconductivity is speculated to exist above the critical temperature TC. Here we show via a combination of far-infrared ellipsometry and ultrafast broadband optical spectroscopy that signatures of such a state can be obtained via three independent observables in an underdoped sample of NdBa2Cu3O6+δ. The pseudogap correlations were disentangled from the...
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