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    Université de Fribourg

    Mapping the unoccupied state dispersions in ${\mathrm{Ta}}_{2}{\mathrm{NiSe}}_{5}$ with resonant inelastic x-ray scattering

    Monney, Claude ; Herzog, Marc ; Pulkkinen, Aki ; Huang, Y. ; Pelliciari, Jonathan ; Olalde-Velasco, P. ; Katayama, Naoyuk ; Nohara, Minoru ; Takagi, Hide ; Schmitt, Thorsten ; Mizokawa, Takashi

    In: Physical Review B, 2020, vol. 102, no. 8, p. 085148

    The transition metal chalcogenide Ta2NiSe5 undergoes a second-order phase transition at Tc=328K involving a small lattice distortion. Below Tc, a band gap at the center of its Brillouin zone increases up to about 0.35 eV. In this work, we study the electronic structure of Ta2NiSe5 in its low-temperature semiconducting phase, using resonant inelastic x-ray scattering (RIXS) at the Ni L3 edge....