Université de Fribourg

Backfolded acoustic phonons as ultrasonic probes in metal-oxide superlattices

Lyzwa, Fryderyk ; Chan, A. ; Khmaladze, Jarji ; Fürsich, K. ; Keimer, B. ; Bernhard, Christian ; Minola, M. ; Mallett, Benjamin P. P.

In: Physical Review Materials, 2020, vol. 4, no. 4, p. 043606

Ultrasonics have been an incisive probe of internal interfaces in a wide variety of systems ranging from stars to solids. For thin-film structures, however, ultrasound is largely ineffective because the signal is dominated by the substrate. Using confocal Raman spectromicroscopy, we show that multiple reflection of sound waves at internal interfaces of a metal-oxide superlattice generates...

Université de Fribourg

Granular superconductivity and charge/orbital order in YBa 2 Cu 3 O 7 /manganite trilayers

Khmaladze, Jarji ; Sarkar, Subhrangsu ; Soulier, Mathias ; Lyzwa, Fryderyk ; Prada, R. de Andres ; Perret, Edith ; Mallett, Benjamin P. P. ; Minola, M. ; Keimer, B. ; Bernhard, Christian

In: Physical Review Materials, 2019, vol. 3, no. 8, p. 084801

We studied how the electronic, superconducting, and magnetic properties of YBa2Cu3O7/Nd1−x(Ca1−ySry )xMnO3 multilayers depend on the tolerance factor and the hole doping of the manganite. In particular, we investigated the granular superconducting state and the related magnetic-field-driven insulator-to- superconductor transition that was previously discovered in corresponding multilayers...

Université de Fribourg

Coupled Cu and Mn charge and orbital orders in YBa₂Cu₃O₇/Nd 0.65 (Ca 1-y Sr y ) 0.35 MnO₃ multilayers

Perret, Edith ; Monney, Claude ; Johnston, S. ; Khmaladze, Jarji ; Lyzwa, Fryderyk ; Gaina, Roxana ; Dantz, M. ; Pelliciari, Jonathan ; Piamonteze, C. ; Mallett, B.P.P. ; Minola, M. ; Keimer, B. ; Schmitt, Thorsten ; Bernhard, Christian

In: Communications Physics, 2018, vol. 1, no. 1, p. 45

The observation of a charge density wave in the underdoped cuprate high Tc superconductors (Cu-CDW) raised a debate about its relationship with superconductivity. In bulk YBa2Cu3O7−δ the Cu-CDW is incipient and mainly pinned by defects. Nevertheless, a large magnetic field can induce a true long-range Cu- CDW order as it suppresses superconductivity. An enhanced Cu-CDW order was also ...

Université de Fribourg

Evidence for spin-triplet superconducting correlations in metal-oxide heterostructures with noncollinear magnetization

Khaydukov, Yu. N. ; Ovsyannikov, G. A. ; Sheyerman, A. E. ; Constantinian, K. Y. ; Mustafa, L. ; Keller, T. ; Uribe-Laverde, Miguel Angel ; Kislinskii, Yu. V. ; Shadrin, A. V. ; Kalaboukhov, A. ; Keimer, B. ; Winkler, D.

In: Physical Review B, 2014, vol. 90, no. 3, p. 035130

Heterostructures composed of ferromagnetic La0.7Sr0.3MnO3, ferromagnetic SrRuO3, and superconducting YBa2Cu3O6+x were studied experimentally. Structures of composition Au/La0.7Sr0.3MnO3/SrRuO3/YBa2Cu3O6+x were prepared by pulsed laser deposition, and their high quality was confirmed by x-ray diffraction and reflectometry. A noncollinear magnetic state of the heterostructures was revealed by means...

Université de Fribourg

Electric-Field-Induced Polar Order and Localization of the Confined Electrons in LaAlO₃/SrTiO₃ Heterostructures

Rössle, Matthias ; Kim, Kyung Wan ; Dubroka, Adam ; Maršík, Premysl ; Wang, Chen Nan ; Jany, R. ; Richter, C. ; Mannhart, J. ; Schneider, C. W. ; Frano, A. ; Wochner, P. ; Lu, Y. ; Keimer, B. ; Shukla, D. K. ; Strempfer, J. ; Bernhard, Christian

In: Physical Review Letters, 2013, vol. 110, no. 13, p. 136805

With ellipsometry, x-ray diffraction, and resistance measurements we investigated the electric-field effect on the confined electrons at the LaAlO₃/SrTiO₃ interface. We obtained evidence that the localization of the electrons at negative gate voltage is induced, or at least enhanced, by a polar phase transition in SrTiO₃ which strongly reduces the lattice polarizability and the subsequent...

Université de Fribourg

Competing interactions at the interface between ferromagnetic oxides revealed by spin-polarized neutron reflectometry

Kim, J.-H. ; Vrejoiu, I. ; Khaydukov, Y. ; Keller, T. ; Stahn, J. ; Rühm, A. ; Satapathy, Dillip Kumar ; Hinkov, V. ; Keimer, B.

In: Physical Review B - Condensed Matter and Materials Physics, 2012, vol. 86, no. 18, p. 180402

We have investigated the magnetization profiles in superlattices composed of the two ferromagnets La0.7Sr0.3MnO₃ and SrRuO₃ using spin-polarized neutron reflectometry. In combination with magnetometry, the neutron data indicate a noncollinear spin configuration where orientation of the Ru moments changes from in plane at the interface to out of plane deep inside the...

Université de Fribourg

Magnetic Proximity Effect in YBa₂Cu₃O₇/La2/3Ca1/3MnO₃ and YBa₂Cu₃O₇/LaMnO₃₊ Superlattices

Satapathy, Dillip Kumar ; Uribe-Laverde, M. A. ; Marozau, I. ; Malik, Vivek K. ; Das, S. ; Wagner, Th. ; Marcelot, C. ; Stahn, J. ; Brück, S. ; Rühm, A. ; Macke, S. ; Tietze, T. ; Goering, E. ; Frañó, A. ; Kim, J. -H. ; Wu, M. ; Benckiser, E. ; Keimer, B. ; Devishvili, A. ; Toperverg, B. P. ; Merz, M. ; Nagel, P. ; Schuppler, S. ; Bernhard, Christian

In: Physical Review Letters, 2012, vol. 108, no. 19, p. 197201

Using neutron reflectometry and resonant x-ray techniques we studied the magnetic proximity effect (MPE) in superlattices composed of superconducting YBa₂Cu₃O₇ and ferromagnetic-metallic La0.67Ca0.33MnO₃ or ferromagnetic-insulating LaMnO₃₊. We find that the MPE strongly depends on the electronic state of the manganite layers, being pronounced for the...

Université de Fribourg

Dimensionality control of electronic phase transitions in nickel-Oxide superlattices

Boris, A. V. ; Matiks, Y. ; Benckiser, E. ; Frano, A. ; Popovich, P. ; Hinkov, V. ; Wochner, P. ; Castro-Colin, M. ; Detemple, E. ; Malik, Vivek Kumar ; Bernhard, Christian ; Prokscha, T. ; Suter, A. ; Salman, Z. ; Morenzoni, E. ; Cristiani, G. ; Habermeier, H.-U. ; Keimer, B.

In: Science, 2011, vol. 332, no. 6032, p. 937-940

The competition between collective quantum phases in materials with strongly correlated electrons depends sensitively on the dimensionality of the electron system, which is difficult to control by standard solid-state chemistry. We have fabricated superlattices of the paramagnetic metal lanthanum nickelate (LaNiO₃) and the wide-gap insulator lanthanum aluminate (LaAlO₃) with atomically...

Université de Fribourg

Evidence of a Precursor Superconducting Phase at Temperatures as High as 180 K in RBa₂Cu₃O7-δ (R=Y,Gd,Eu) Superconducting Crystals from Infrared Spectroscopy

Dubroka, Adam ; Rössle, Matthias ; Kim, Kyung Wan ; Malik, Vivek Kumar ; Munzar, Dominik ; Basov, D. N. ; Schafgans, A. A. ; Moon, S. J. ; Lin, C. T. ; Haug, D. ; Hinkov, V. ; Keimer, B. ; Wolf, Th. ; Storey, J. G. ; Tallon, Jeffery L. ; Bernhard, Christian

In: Physical Review Letters, 2011, vol. 106, no. 4, p. 047006

We show that a multilayer analysis of the infrared c-axis response of RBa₂Cu₃O7-δ (R=Y,Gd,Eu) provides important new information about the anomalous normal-state properties of underdoped cuprate high temperature superconductors. In addition to competing correlations which give rise to a pseudogap that depletes the low-energy electronic states below...