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    Université de Fribourg

    Nonthermal excitonic condensation near a spin-state transition

    Werner, Philipp ; Murakami, Yuta

    In: Physical Review B, 2020, vol. 102, no. 2020-24, p. 241103

    Recent experiments demonstrate the induction of long-range order in correlated electron systems via external perturbations, which calls for a better understanding of nonthermal ordered states and nonequilibrium symmetry breaking. Here, we reveal a mechanism based on entropy cooling and entropy trapping in a strongly correlated multiorbital system. We consider a two-orbital Hubbard model with...

    Université de Fribourg

    NESSi : The Non-Equilibrium Systems Simulation package

    Schüler, Michael ; Golež, Denis ; Murakami, Yuta ; Bittner, Nikolaj ; Herrmann, Andreas ; U.R.Strand, Hugo ; Werner, Philipp ; Eckstein, Martin

    In: Computer Physics Communications, 2020, vol. 257, no. 2020, p. 107484

    The nonequilibrium dynamics of correlated many-particle systems is of interest in connection with pump–probe experiments on molecular systems and solids, as well as theoretical investigations of transport properties and relaxation processes. Nonequilibrium Green’s functions are a powerful tool to study interaction effects in quantum many-particle systems out of equilibrium, and to extract...

    Université de Fribourg

    High-harmonic generation in spin-orbit coupled systems

    Lysne, Markus ; Murakami, Yuta ; Schüler, Michael ; Werner, Philipp

    In: Physical Review B, 2020, vol. 102, no. 8, p. 081121

    We study high-harmonic generation in two-dimensional electron systems with Rashba and Dresselhaus spin-orbit coupling and derive harmonic generation selection rules with the help of group theory. Based on the band structures of these minimal models and explicit simulations we reveal how the spin-orbit parameters control the cutoff energy in the high-harmonic spectrum. We also show that the...

    Université de Fribourg

    Signatures of bosonic excitations in high-harmonic spectra of Mott insulators

    Lysne, Markus ; Murakami, Yuta ; Werner, Philipp

    In: Physical Review B, 2020, vol. 101, no. 19, p. 195139

    The high-harmonic spectrum of the Mott insulating Hubbard model has recently been shown to exhibit plateau structures with cutoff energies determined by nth-nearest- neighbor doublon-holon recombination processes. The spectrum thus allows one to extract the on-site repulsion U. Here, we consider generalizations of the single-band Hubbard model and discuss the signatures of bosonic excitations...

    Université de Fribourg

    Collective modes in excitonic insulators: Effects of electron-phonon coupling and signatures in the optical response

    Murakami, Yuta ; Golež, Denis ; Kaneko, Tatsuya ; Koga, Akihisa ; Millis, Andrew J. ; Werner, Philipp

    In: Physical Review B, 2020, vol. 101, no. 19, p. 195118

    We consider a two-band spinless model describing an excitonic insulator (EI) on the two-dimensional square lattice with anisotropic hopping parameters and electron-phonon (el-ph) coupling, inspired by the EI candidate Ta2NiSe5. We systematically study the nature of the collective excitations in the ordered phase which originates from the interband Coulomb interaction and the el-ph coupling. ...

    Université de Fribourg

    Ultrafast nonequilibrium evolution of excitonic modes in semiconductors

    Murakami, Yuta ; Schüler, Michael ; Takayoshi, Shintaro ; Werner, Philipp

    In: Physical Review B, 2020, vol. 101, no. 3, p. 035203

    We study the time evolution of excitonic states after photoexcitation in the one- dimensional spinless extended Falicov-Kimball model. Several numerical methods are employed and benchmarked against each other: time-dependent mean-field simulations, the second-Born approximation (2BA) within the Kadanoff-Baym formalism, the generalized Kadanoff-Baym ansatz (GKBA) implemented with the 2BA, and...

    Université de Fribourg

    Quantum simulation meets nonequilibrium dynamical mean-field theory: exploring the periodically driven, strongly correlated fermi-hubbard model

    Sandholzer, Kilian ; Murakami, Yuta ; Görg, Frederik ; Minguzzi, Joaquín ; Messer, Michael ; Desbuquois, Rémi ; Eckstein, Martin ; Werner, Philipp ; Esslinger, Tilman

    In: Physical Review Letters, 2019, vol. 123, no. 19, p. 193602

    We perform an ab initio comparison between nonequilibrium dynamical mean-field theory and optical lattice experiments by studying the time evolution of double occupations in the periodically driven Fermi-Hubbard model. For off-resonant driving, the range of validity of a description in terms of an effective static Hamiltonian is determined and its breakdown due to energy absorption close to...

    Université de Fribourg

    High-harmonic generation in quantum spin systems

    Takayoshi, Shintaro ; Murakami, Yuta ; Werner, Philipp

    In: Physical Review B, 2019, vol. 99, no. 18, p. 184303

    We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by ac electric fields produces radiation from the dynamics of excited charges, we consider here the situation where spin systems excited by a magnetic field pulse generate radiation via a time- dependent magnetization. Specifically, we study the magnetic dipole...

    Université de Fribourg

    Nonequilibrium steady states of electric field driven Mott insulators

    Murakami, Yuta ; Werner, Philipp

    In: Physical Review B, 2018, vol. 98, no. 7, p. 075102

    We present a systematic study of the nonequilibrium steady states (NESS) in Mott insulators driven by dc or ac electric fields, based on the Floquet dynamical mean- field theory. The results are analyzed using a generalized tunneling formula for the current, which is reminiscent of the Meir-Wingreen formula and provides insights into the relevant physical processes. In the dc case, the...

    Université de Fribourg

    High-harmonic generation in Mott insulators

    Murakami, Yuta ; Eckstein, Martin ; Werner, Philipp

    In: Physical Review Letters, 2018, vol. 121, no. 5, p. 057405

    Using Floquet dynamical mean-field theory, we study the high-harmonic generation in the time-periodic steady states of wide-gap Mott insulators under ac driving. In the strong-field regime, the harmonic intensity exhibits multiple plateaus, whose cutoff energies εcut=U+mE0 scale with the Coulomb interaction U and the maximum field strength E0. In this regime, the created doublons and holons...